Kinetic Monte Carlo simulation of irradiation-induced nanostructure evolution in Oxide Dispersion Strengthened Fe alloys


Kinetic Monte Carlo simulation of irradiation-induced nanostructure evolution in Oxide Dispersion Strengthened Fe alloys

Liedke, B.; Posselt, M.; Murali, D.; Claisse, A.; Olsson, P.

Rigid-lattice Kinetic Monte Carlo simulations are performed in order to investigate the modification of Y-Ti-O nanoclusters during irradiation, at selected temperatures, doses and dose rates. The simulations use input parameters for the atomic interactions and the migration barriers obtained by DFT calculations as well as data on representative examples of the cascade debris determined by Molecular Dynamics. Before irradiation the nanostructure is prepared by performing thermal relaxation of a system with randomly distributed Y, Ti, O atoms, and vacancies. The concentration of Y, Ti, and O is chosen according to the common 14 YWT ODS alloy and both low and high vacancy contents are considered. The nanostructures obtained in the preparation step were used subsequently in KMC simulations of irradiation. The results demonstrate the competition between ballistic effects leading to the dissolution and the growth of the clusters. While the former effect dominates at high doses and low temperatures the latter prevails at low doses and high temperatures. On the other hand, the nanoclusters formed in the preparation step show a very high stability under irradiation within the temperature and dose range relevant for the application of ODS alloys in advanced nuclear reactors. The findings of this work are consistent with the results of experimental studies of ion and neutron irradiation of ODS alloys.

Keywords: Oxide Dispersion Strengthened (ODS) Fe alloys; Kinetic Monte Carlo simulation; Irradiation

  • Lecture (Conference)
    13th International Conference on Computer Simulation of Radiation Effects in Solids (COSIRES 2016), 19.-24.06.2016, Loughborough, UK

Permalink: https://www.hzdr.de/publications/Publ-23875
Publ.-Id: 23875