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The Crystal Electric Field Effect in the Distorted Kagome Lattice Ferromagnet Nd3Ru4Al12

Ishii, I.; Mizuno, T.; Kumano, S.; Umeno, T.; Suzuki, D.; Andreev, A. V.; Gorbunov, D.; Henriques, M. S.; Suzuki, T.
The distorted kagome lattice compound Nd3Ru4Al12 shows a ferromagnetic phase transition at TC =39 K. Reduced Nd magnetic moments with two different values of 2.66 and 0.95 µB are aligned along the c-axis below TC. It was previously reported that a crystal electric field (CEF) effect may affect the reduced magnetic moments. To clarify the 4f -electronic state in Nd3Ru4Al12, we performed CEF analyses for the inverse magnetic susceptibility and magnetization. We proposed the CEF level scheme of which the inverse magnetic susceptibilities along both a- and c-axes are reproduced. The ferromagnetic phase transition at TC along the c-axis can be explained by a simple CEF model. In contrast, reduced magnetic moments cannot be understood by the simple CEF model, because calculated magnetization curves are quite larger than the experimental data.
  • Contribution to proceedings
    International Conference on Strongly Correlated Electron Systems (SCES2019), 23.-28.09.2019, Okayama, Japan
    JPS Conference Proceedings 30(2020), 011161
    DOI: 10.7566/JPSCP.30.011161

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Permalink: https://www.hzdr.de/publications/Publ-30849
Publ.-Id: 30849