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Nonlinear IR and THz Spectroscopy of Semiconductor Nanowires

Helm, M.; Fotev, I.; Balaghi, L.; Lang, D.; Rana, R.; Winnerl, S.; Schneider, H.; Dimakis, E.; Pashkin, A.

We report nonlinear charge-carrier response in GaAs/InGaAs core/shell nanowires that are driven by intense THz pulses. In the first experiment, half-cycle THz pulses emitted from an organic DSTMS crystal lead to a red-shift of the plasmon Peak indicating intervalley transfer of the electrons. In the second experiment, a single, highly electron doped nanowire is investigated by scattering near-field infrared microscopy using intense free-electron laser (FEL) pulses. Here the observed red shift of the mid-infrared plasma resonance depends on the pulse energy and can be explained by heating the electron system in the nonparabolic conduction band.

Keywords: nanowire; THz; infrared; free-electron laser; near-field microscopy; nonlinear

  • Invited lecture (Conferences) (Online presentation)
    45th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz 2020), 08.-13.11.2020, Buffalo, USA

Permalink: https://www.hzdr.de/publications/Publ-31719
Publ.-Id: 31719


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