Department of Reactive Transport
In the Reactive Transport Department we study the heterogeneity of material surface reactivity, including sorption and dissolution reactions and material degradation. We use experimental and numerical methods to quantify and predict surface reaction rates using rate maps. Transport in complex porous materials is another important aspect of our work. We develop conservative and reactive radionuclide tracers using our cyclotron laboratory and apply positron emission tomography (PET). We use and develop numerical methods for transport analysis at the pore scale and above. Our research is motivated and driven by applications in nuclear safety research and we provide critical links to earth, environmental and materials sciences.
Latest publication
Cyclotron production and purification of 83Sr as a 90Sr substitute for Positron Emission Tomography (PET)
Lindemann, M.; Schöngart, J.; Štursa, J.; Franke, K.
Abstract
Radioactive contaminations in soil, which originate from nuclear power production, nu-clear weapon testing or uncontrolled release, are of great environmental concern. One of the major fission product contaminants is 90Sr, whose high mobility demands a method to track contamination pathways and remediation processes. Positron emission tomography (PET) is a valuable tool for the required studies. As a β-/γ-emitter, 90Sr is not suitable for PET, which requires β+-emitters. As an alternative, 83Sr offers, with a 12% intensity of β+-emission and a half-life of 32.4 h an appropriate PET substitute for 90Sr. We produced 83Sr with an enriched target of [85Rb]RbCl in an 85Rb(p,3n)83Sr reaction. The target material was bombarded with 36.22 MeV protons (ø 2 µA, 315 min), at a solid target station at the cyclotron U-120M (NPI CAS). The irradiated target (1.5 GBq) was dissolved in water, evaporation to dryness, redissolved in nitric acid and transferred onto a Sr-selective car-tridge (Sr-SpecTM, TRISKEM, France). Following target material wash out, 83Sr elution with water, solvent evaporation and reformulation (dilute nitric acid) yielded 1.2 GBq (82% radiochemical extraction efficiency, non-decay corrected) of an 83Sr-solution. The easy and fast method is able to produce non-carrier-added 83Sr with high radionuclidic purity.
Keywords: 83Sr; Strontium-83; Rubidium-85; Rubidium target; cyclotron; PET
Related publications
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Cyclotron production and purification of 83Sr as a 90Sr substitute for …
ROBIS: 42922 HZDR-primary research data are used by this (Id 42867) publication
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Instruments 10(2026)2, 20
DOI: 10.3390/instruments10020020
Permalink: https://www.hzdr.de/publications/Publ-42867
Team
Head/ Administration | |||||
| Name | Bld./Office | +49 351 260 | Position/Tasks | ||
|---|---|---|---|---|---|
| Prof. Dr. Cornelius Fischer | L9.3/212 | 4660 | c.fischer | Head of Department | |
| Katrin Gerstner | L9.3/217 | 4601 | k.gerstner | Secretary's office / Administration Reactive Transport / Experimental Neurooncological Radiopharmacy | |
| Nadja Pedrosa Gil | L9.3/221 | 4690 | n.pedrosa-gil | Business administration Reactive Transport & Business administration Experimental Neurooncological Radiopharmacy 2 nd Deputy of the Equal Opportunity Officer | |
Employees | |||||
| Name | Bld./Office | +49 351 260 | Position/Tasks | ||
| Sieglinde Holzknecht | L9.3/222 | 4664 | s.holzknecht | PhD Student | |
| Dr. Johannes Kulenkampff | L9.3/202 | 4663 | j.kulenkampff | Research Scientist | |
| Dr. Marcel Lindemann | L9.3/318 | 4671 | m.lindemann | Research Scientist | |
| Dr. habil. Holger Lippold | L9.3/401 | 4672 | h.lippold | Research Scientist | |
| Dagmar Lösel | L9.3/402 | 4673 | d.loesel | Laboratory technician | |
| Jann Schöngart | L9.3/222 | 4658 | j.schoengart | Research Scientist | |
| Claudia Schößler | L9.3/402 | 4674 | c.schoessler | Chemical laboratory technician | |
Other employees | |||||
| Name | Bld./Office | +49 351 260 | Position/Tasks | ||
| Dr. Karsten Franke | L9.3/318 | 4629 | k.franke | Research Associate | |
