Non-Equilibrium Warm Dense Matter
Research on properties of matter as in the centre of planets or stars, created by short- and long pulse lasers, x-rays, ion or electron beams, in diamond anvil cells or for fusion energy production.
Ion acoustic modes in liquids and plasmas are equivalent to phonons in solids. They play an important role for energy transfer processes during temperature relaxation, influence the stopping of fast particles, and allow to determine the speed of sound in the medium as well as the temperature (via detailed balance). Our theoretical understanding of ion acoustic modes is crucial for our capabilities to model and interpret the x-ray scattering signal in experiments and to investigate new states of matter. Here, we (P. Mabey und Kollegen aus Oxford, Kollegen von SLAC/SIMES) investigated ion acoustic modes using first principle simulations.
Laser irradiation of metals creates non-equilibrium states with high energy electrons. The relaxation in the system and the coupling to the phonons is a complicated process that sometimes is modelled within a two-temperature model. We (R. Ernstorfer and colleagues from FHI Berlin) found that a much better description is given by including the non-thermal behaviour of the phonons.
Shock-compressed carbon changes phase from graphite to diamond. Under certain conditions, hexagonal diamond -lonsdaleite- can be produced. Lonsdaleite is a metastable phase of carbon featuring a crystal lattice structure in between graphite and diamond. Calculations predict lonsdaleite to be harder than diamond. Naturally occuring londsaleite is possibly generated in meteorite impacts. A collaboration under principal investigator Dominik Kraus (HZDR, University Berkeley) has just published these new insights. There is a nice summary here.
Gitter- und Elektronenstruktur in warmem Diamant bei p=130GPa (links), in warmem Lonsdaleite bei p=200GPa (mitte) und in flüssigem Kohlenstoff bei p=150GPa (rechts).
We are using first principle simulations like density functional molecular dynamics and quantum statistical Green's function methods to describe new and exotic states of matter in equilibrium and non-equilibrium and during various relaxation processes. We give predictions for x-ray spectra that may be obtained by scattering experiments.
Molecular hydrogen as in Jupiter's outer mantle, warm dense aluminium created by laser generated shock waves, metallic hydrogen as in Jupiters core.