Nuclear Physics

Modern accelerator mass spectrometry is a technique, which was born in nuclear physics laboratories in the late seventies of the last century. Many different research areas are touched by AMS, including archaeology, biological applications, atmospheric science, climatology, environmental science, hydrology, oceanography, glaciology, geological applications, nuclear forensics, ice core research, astrophysics, cosmic-rays, meteorites, nuclear physics and particle physics.

Applications

Chart of Nuclides ©Edward Simpson, https://people.physics.anu.edu.au/~ecs103/chart

The Colourful Nuclide Chart: Edward Simpson, https://people.physics.anu.edu.au/~ecs103/chart

Half-live measurements. Half-life values are a fundamental nuclear physics quantity for dating applications where the decay in combination with its half-life value is used (note, the situation is different for 14C where an absolute time calibration independent of the half-life value has been established). The half-life is often also directly related to the isotope ratio of AMS standards, because the absolute number of the radionuclide in a sample can be deduced from its activity and the half-life value. New state-of-the-art AMS systems can produce highly precise data, e.g. 10Be/9Be ratios can be measured to better than 1%. Therefore, also the standards and consequently half-life values need to be known accurately. AMS had been used to measure half-lives of long-lived radionuclides, e.g. 32Si, 41Ca, 60Fe or 146Sm.

Island of stability ©Yuri Organessian

In this illustration, the ships represent the chemical reactions used to reach the "island of stability" of superheavy elements.

Search for super-heavy elements in nature. The discovery of new elements (natural or artificially produced) has been a driving force in chemistry and physics. A run for the search for long-lived superheavy elements, possibly present in Nature since the formation of the solar system, started shortly after the hypothesis of an island of stability was suggested. Such species could be produced in nucleosynthesis by the rapid (r-) neutron capture process, as is the case in our present understanding for naturally occurring thorium and uranium. Similar to the search for interstellar longer-lived radionuclides in terrestrial archives (see Astrophysics and Meteorites), AMS is also used for direct search of such exotic nuclides. So far, no evidence exists and AMS measurements reached limits of abundance sensitivity in the 10-12 to 10-16 range relative to stable chemical homologues.

U and Pu production

Production of the major actinide nuclides through neutron capture reactions

Nucleosynthesis in the laboratory—nuclear reaction studies. The knowledge of nuclear reaction cross sections has always been a prime goal of experimental nuclear physics. Nuclear data are of crucial importance in many applications - AMS represents a complementary approach for the precise measurements of cross sections (see also Astrophysics and Meteorites). Such applications include nuclear astrophysics (nucleosynthesis, cosmo-chemistry, meteorites), space technology, nuclear technology (nuclear fusion, nuclear fission and advanced reactor concepts) and medical applications (hadron therapy, radiation dose measurements). Furthermore, many applied AMS research areas rely on a proper understanding of the production of cosmogenic radionuclides in environmental, geological and extraterrestrial studies. Cross-sections and total induced activities are key parameters for safety and design analyses in advanced reactor concepts, such as fusion applications; i.e. accurate cross sections are crucial for calculating the production of long-lived activation products. In a fusion environment, particularly long-lived activation products may lead to significant long-term waste disposals and radiation damage.

ITER Tokamak and Plant Systems ©Oak Ridge National Laboratory

ITER Tokamak and Plant Systems (Oak Ridge National Laboratory)

This work relates to ITER, generation IV reactors, advanced reactor concepts, accelerator driven systems, and accelerators for medical applications. These research activities include a number of collaborations, e.g. with JRC/IRMM (Joint European Centre, Geel, Belgium), IAEA (Vienna), VERA (Univ. of Vienna) and ANSTO/Sydney; FRM II/TU Munich, ILL/Grenoble and Atominstitut – TU Vienna. We are linked to the IAEA through specialist’s activities within their nuclear data program. We are also part of the n_TOF collaboration through complementary measurements. n_TOF is a pulsed neutron source at CERN and designed to study neutron-induced interactions for neutron energies between meV to GeV. Research fields range from stellar nucleosynthesis to applications of nuclear technology, including the transmutation of nuclear waste and accelerator driven systems.

NaI crystal ©M.A. Oliván Light yield determination in large sodium iodide detectors applied in the search for dark matter, Astroparticle Physics 2017

A 10.7 kg hexagonal prism NaI(Tl) crystal

Radioimpurities in particle detectors for dark matter studies. AMS allows to study extremely low levels of radioactivity in ultra-high purity detector materials that need to be characterized for Dark Matter studies. We are part of the SABRE-South collaboration through the Australian Centre of Excellence for Dark Matter Particle Physics. SABRE (Sodium iodide with Active Background Rejection) is designed as a dark matter direct detection system to be installed in an underground laboratory in Australia.

Measurement of the neutrino mass. 163Ho (T1/2 = 4570 yr) is an interesting candidate for studying the mass scale of the electron neutrino. The main reason is its very low-energy electron-capture decay properties. Crucial for this study is the production of a sample containing 163Ho of sufficient activity combined with high isotopic purity (see ECHO project). A major concern in this respect is the co-production of another long-lived isotope 166mHo (T1/2 = 1200 yr). AMS is used to verify the isotopic purity of 163Ho and to quantify 166mHo impurities.


User Information

see here

Projects and Collaborations

Further Reading

Fundamentals

  • W. Kutschera and M. Paul (1990), Accelerator mass spectrometry in nuclear physics and astrophysics, Annu. Rev. Nucl. Part. Sci. 40, 411-438.
  • L.Gastaldo et al., The electron capture in 163Ho experiment – ECHo Eur. Phys. J. Spec. Top. 226, 1623-1694 (2017)
  • M. Antonello et al., (The SABRE collaboration), The SABRE project and the SABRE Proof-of-Principle. https://arxiv.org/abs/1806.09340, The European Physical Journal C79 (2019) 363.

Own publications (see also here)

  • Wallner, A., Bichler, M., Buczak, K., Dillmann, I., Käppeler, F., Karakas, A., Lederer, C., Lugaro, M., Mair, K., Mengoni, A., Schätzel, G., Steier P. and Trautvetter, H.P. (2016). Accelerator mass spectrometry measurements of the 13C(n,γ)14C and 14N(n,p)14C cross sections. Phys. Rev. C93, 045803. https://doi.org/10.1103/PhysRevC.93.045803
  • Damone, L. et al. (The n_TOF collaboration) (2018). The 7Be(n,p)7Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN). Physical Review Letters 121, 042701. https://doi.org/10.1103/PhysRevLett.121.042701
  • Gyürky, Gy., Fülöp, Zs., Käppeler, F., Kiss, G.G. and Wallner, A. (2019). The activation method for cross section measurements in nuclear astrophysics. Review, Europ. Phys. Journal A 55, 41.