Spin dynamics of NiCl2-4SC(NH2)2 in the field-induced ordered phase


Spin dynamics of NiCl2-4SC(NH2)2 in the field-induced ordered phase

Zvyagin, S.; Wosnitza, J.; Kolezhuk, A. K.; Zapf, V. S.; Jaime, M.; Paduan-Filho, A.; Glazkov, V. N.; Sosin, S. S.; Smirnov, A. I.

NiCl2-4SC(NH2)2 (known as DTN) is a spin-1 material with a strong single-ion anisotropy that is regarded as a new candidate for Bose-Einstein condensation (BEC) of spin degrees of freedom. We present a systematic study of the low-energy excitation spectrum of DTN in the field-induced magnetically ordered phase by means of high-field electron spin resonance measurements at temperatures down to 0.45 K. We argue that two gapped modes observed in the experiment can be consistently interpreted within a four-sublattice antiferromagnet model with a finite interaction between two tetragonal subsystems and unbroken axial symmetry. The latter is crucial for the interpretation of the field-induced ordering in DTN in terms of BEC.

  • Physical Review B 77(2008), 092413

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