Evidence for an Fulde-Ferrell-Larkin-Ovchinnikov State with Segmented Vortices in the BCS-BEC-Crossover Superconductor FeSe

We present resistivity and thermal-conductivity measurements of superconducting FeSe in intense magnetic fields up to 35 Tapplied parallel to the ab plane. At low temperatures, the upper critical field μ₀H^ab _c2 shows an anomalous upturn, while thermal conductivity exhibits a discontinuous jump at μ₀H* ≈ 24 T well below μ₀H^ab _c2, indicating a first-order phase transition in the superconducting state. This demonstrates the emergence of a distinct field-induced superconducting phase. Moreover, the broad resistive transition at high temperatures abruptly becomes sharp upon entering the high-field phase, indicating a dramatic change of the magnetic-flux properties.We attribute the high-field phase to the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state, where the formation of planar nodes gives rise to a segmentation of the flux-line lattice. We point out that strongly orbital-dependent pairing as well as spin-orbit interactions, the multiband nature, and the extremely small Fermi energy are important for the formation of the FFLO state in FeSe.