CyClotron "CYCLONE 18/9"
The department of Reactive Transport in Leipzig utilizes the cyclotron CYCLONE 18/9® (Ion Beam Applications, IBA, Belgian) for the generation of radionuclides needed in the ongoing research. This particle accelerator supplies protons with an energy of 18 MeV and deuterons with an energy of 9 MeV and enables (p,x) and (d,x) – nuclear reactions. Two internal ion sources generate negatively charged hydrogen and deuteron ions, which are accelerated and after passing stripper foils are guided as protons and deuterons to the eight possible beam exits. A possible beam splitting enables the irradiation of two beam exits simultaneously. The maximum extractable beam current on target is 100 µA for protons and 40 µA for deuterons.
The eight beam exits are equipped with target stations for the irradiation of gaseous targets (e.g. generation of [11C]CO2, [11C]CH4 and [15O]O2), liquid targets (e.g. generation of [18F]F2)) and solid targets. COSTIS 1 and COSTIS 2 are the two available target station for the irradiation of solid targets. COSTIS 1 allows the irradiation of target capsules (diameter = 24 mm, thickness = 5 mm) and is utilized for the irradiation of powders, like oxides, nanoparticles (NP) and salts. COSTIS 2 handles disc-like targets (diameter = 24 mm, thickness = 2 mm) for the irradiation of foils and electroplated samples.
Established nuclear reactions in solid targets
Nuclear reaction | Target material | Parameters | Applications |
---|---|---|---|
natLi(p,n)7Be | LiH / nanoparticles (MWCNT) |
Ep = 2.5 MeV Ip = 5 µA |
Nanosafety research [7Be]MWCNT |
natMg(d,α)22Na | Mg-foil 300 µm |
Ed = 8.9 MeV Id = 10 µA |
Tracer for transport studies (PET) |
natSc(p,n)45Ti |
Sc-foil |
Ed = 12 MeV Id = 20 µA |
Nanosafety research (TiO2-NP) |
natTi(p,n)48V |
Ti-foil |
Ep = 12 MeV |
Material recycling of metallurgic slags |
natTi(p,n)48V |
TiO2-NP |
Ep = 12 MeV Ip = 7.5 µA |
Nanosafety research [48V]TiO2 |
natV(p,n)51Cr | V-foil 127 µm |
Ep = 11 MeV Ip = 20 µA |
Recycling (stainless steel slags, ferrochrome slags) |
natFe(p,n)56Co | Fe-foil 100 µm |
Ep = 13.4 MeV Ip = 22 µA |
Tracer for transport studies (PET) |
64Ni(p,n)64Cu | 64Ni-clectro plate | Ep = 12 MeV Ip = 22 µA |
Tracer for transport studies (PET) |
natRb(p,n)85Sr | RbCl pellet 300 µm |
Ep = 13.4 MeV Ip = 5 µA |
Nuclear waste research (90Sr-analog) |
natSr(p,n)88Y | SrCO3 pellet 300 µm |
Ep = 12 MeV Ip = 3 µA |
Y as analog for REE in transport studies / extraction studies |
natY(p,n)89Zr | Y-foil 150 µm |
Ep = 12 MeV Ip = 22 µA |
REE ore leaching, Zr as major contaminant |
natZr(d,n)95Nb | Zr-foil 127 µm |
Ed = 9 MeV Id = 10 µA |
Tracer for transport studies |
135Ba(p,n)135La | [135Ba]BaCO3 pellet 600 µm |
Ep = 18 MeV Ip = 12.5 µA |
Ore chemistry, separation of Lanthanides |
natLa(p,n)139Ce | La2O3 pellet 300 µm |
Ep = 12.5 MeV Ip = 22 µA |
Ore chemistry, separation of Lanthanides |
natCe(p,2n)139Pr | CeO2-NP | Ep = 18 MeV Ip = 7.5 µA |
Nanosafety research |