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Neue Rechnungen zu Lufteinbruchstörfällen bei Fusionsreaktoren mit einer Beschichtung des Reaktorraums aus CFC-Material
Krüssenberg, A.-K.; Hicken, E. F.
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Contribution to proceedings
Jahrestagung Kerntechnik 1998 S. 573-576 -
Lecture (Conference)
Jahrestagung Kerntechnik 1998, 26.-28.5.1998, München
Permalink: https://www.hzdr.de/publications/Publ-1050
Publ.-Id: 1050
Stickstofftransport während der plasmagestützten Randaufstickung nichtrostender Stähle - der Einfluß der passivierenden Oxidschicht
Parascandola, S.; Kruse, O.; Richter, E.; Möller, W.
Plasmagestütztes Randaufsticken ist eine erfolgversprechende Technologie zur Verbesserung der Verschleiß- und der Korrosionseigenschaften von Bauteilen aus nichtrostendem Stahl. Bei moderaten Temperaturen (ca. 400°C) kann eine Randschicht mit einem hohem Gehalt an gelöstem Stickstoff (ca. 20at.%) erzeugt werden. Diese Randschicht weist eine deutlich erhöhte Härte und Verschleißbeständigkeit und eine hervorragende Korrosionsbeständigkeit auf. Die Prozesse, die zur Bildung dieser Randschicht führen, sind weitgehend unverstanden. Um den Einfluß der passivierenden Oxidschicht auf die Bildung der stickstoffreichen Randschicht zu untersuchen, ist ein in-situ Experiment mit einer gekreuzten Strahlgeometrie aufgebaut worden. Bei kontrollierten Restgaszusammensetzungen wird während des plasmagestützten Randaufstickens zeit- und tiefenaufgelöste Elementanalyse betrieben. Dabei wird zum Randaufsticken eine Hochstrom-Ionenquelle und zur tiefenaufgelöste Elementanalyse „elastic recoil detection analysis“ (ERDA) verwendet. ERDA ist sensitiv auf die leichten Elemente und wurde hier hinsichtlich schneller Datenaufnahme optimiert. Quantitative zeitaufgelöste Messungen der Elementverteilungen werden für verschiedene Sauerstoffpartialdrücke vorgestellt. Die Bildung der stickstoffreichen Randschicht ist stark mit der Reduzierung der Oxidschicht korreliert. Hohe Sauerstoffpartialdrücke stabilisieren die Oxidschicht. Dieses Ergebnis stimmt gut überein mit einem einfachen Transportmodell, das die Sauerstoffadsorptionsrate und die Zerstäubungsrate berücksichtigt.
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Lecture (Conference)
Nichtmetalle in Metallen: Tagung des Gemeinschaftsausschusses "Nichtmetalle in Metallen" der GDMB, 23-25 März 1998 in Münster / Nichtmetalle in Metallen '98: Vortragstexte einer Tagung des Gemeinschaftsausschusses "Nichtmetalle in Metallen" der G... -
Contribution to proceedings
Nichtmetalle in Metallen: Tagung des Gemeinschaftsausschusses "Nichtmetalle in Metallen" der GDMB, 23-25 März 1998 in Münster / Nichtmetalle in Metallen '98: Vortragstexte einer Tagung des Gemeinschaftsausschusses "Nichtmetalle in Metallen" der G...
Permalink: https://www.hzdr.de/publications/Publ-1049
Publ.-Id: 1049
Härtung von Edelstahl durch Stickstoff-Plasma-Immersions-Ionenimplantation
Richter, E.; Günzel, R.
- Ingenieur-Werkstoffe 6 (1997) 44
Permalink: https://www.hzdr.de/publications/Publ-1046
Publ.-Id: 1046
Noise Analysis Measurements and Numerical Evaluations of the Moderator Temperature Coefficient in PWRs
Laggiard, E.; Grundmann, U.; Rohde, U.; Weiß, F.-P.; Runkel, J.; Stegemann, D.
The moderator temperature coefficient (MTC) of a 1400 MW pressurized water reactor (PWR) has been measured from neutron and temperature fluctuations in different reactor positions. In order to explain the deviations observed between the estimations, numerical evaluations of the MTC were performed using the 3D two energy groups DYN3D code for a prototype PWR. The differences between the experimental MTC estimations can be partially explained considering that the numerical MTC evaluations show a definite devitation of the neutronics from point kinetics.
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Other report
27th Informal Meeting on Reactor Noise (IMORN 27), Valencia, November 18 - 20, 1997 -
Lecture (Conference)
27th Informal Meeting on Reactor Noise (IMORN 27), Valencia, November 18 - 20, 1997
Permalink: https://www.hzdr.de/publications/Publ-1045
Publ.-Id: 1045
Nicotinamide-Substituted Complexes as Redox Marker
Knieß, T.; Spies, H.; Brandau, W.; Johannsen, B.
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Journ. Labelled Comp. and Radiopharm. XLI, 605-614 (1998)
DOI: 10.1002/(SICI)1099-1344(199807)41:7<605::AID-JLCR112>3.0.CO;2-P
Cited 7 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1044
Publ.-Id: 1044
Annealing studies of chromium implanted silicon nitride ceramics
Brenscheidt, F.; Matz, W.; Wieser, E.; Möller, W.
The effect of chromium implantation and subsequent annealing
on the hardness and wear behaviour of a silicon nitride-based ceramic is
investigated. Implantation energies were 200, 400, 1000 and 2000 keV, the
fluence was 1017 Cr+ ions cm-2 in all cases. The annealing temperatures
were 800 C, 1000 C and 1200 C. The phase composition was determined with
X-ray diffraction. Annealing at 800 C does not affect the crystal structure.
At 1000 C the -Si3N4-phase is formed for 1 and 2 MeV implantation energy.
At 1200 C, Cristobalite and Keiviite are formed at the lower implantation
energies; at higher energies -Si3N4 is formed. We discuss the phase formation
for the different implantation energies and annealing temperatures and
the relationship with the observed hardness and wear.
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Nuclear Instruments and Methods in Physics Research B 127/128 (1997) 677-680
DOI: 10.1016/S0168-583X(96)01154-8
Cited 6 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1043
Publ.-Id: 1043
Surface Roughness with Nanometer-Scale Ag Particles Generated by Ion Implantation
Pham, M. T.; Matz, W.; Seifarth, H.
Surfaces of SiO2, Si3N4, Ta2O5 and glass were implanted
with Ag+ ions. Studies using X-ray diffraction (XRD) and atomic force microscopy
(AFM) show that the surface morphology is dominated by metallic silver
features consisting of regularly shaped, mostly spherical, Ag particles
spanning a size range from some nanometers to some 100 nm in diameter.
The particle size metrics, distribution, shape, and their density are shown
to be controlled by the process paramters ion dose, dose rate, and ion
energy. Adjusting the energy of the incident ions results in various degrees
of submerging into the substrate including exposed Ag features anchored
onto the surface or buried Ag particles overcoated by a thin layer of the
matrix material. The substrate material differs by its ability of stabilizing
the dispersion and blocking the Ag movement. Ta2O5 and glass substrates
provide more homogeneously dispersed Ag particles, much smaller in size
and regularly shaped compared to SiO2 and Si3N4 substrate systems. Potential
application refers to surface enhanced Raman scattering.
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Analytica Chimica Acta 350 (1997) 209-220
DOI: 10.1016/S0003-2670(97)00294-8
Cited 18 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1042
Publ.-Id: 1042
Comparison of Computer Generated and ERDA depth Profiles of Oxygen Implanted into Silicon with Plasma Immersion Ion Implantation
Barradas, N. P.; Maas, A. J. H.; Mändl, S.
Plasma immersion ion implantation was used to implant
oxygen into silicon with nominal doses ranging from 2 x 1016 to 2 x 1017/cm2.
Positive Ions, O+2 and O+, with a continuous energy distribution between
0 and 40 keV were implanted. The plasma parameters and the geometrical
configuration of the implantation were chosen in order to follow closely
the assumptions of a theoretical model, which allowed to calculate the
energy distribution of the incident ions. Computer simulations were performed
to derive the resulting theoretical oxygen depth distribution. The agreement
found with the experimental depth profiles, measured by elastic recoil
detection analysis, is good. The small discrepancy observed is discussed
in terms of the shortcomings of the model used.
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Nuclear Instruments and Methods in Physics Research B 124 (1997) 63-68
DOI: 10.1016/S0168-583X(97)00102-X
Permalink: https://www.hzdr.de/publications/Publ-1041
Publ.-Id: 1041
Quality assurance of heavy ion tumour therapy by means of positron emission tomography.
Enghardt, W.; Debus, J.; Hasch, B.-G.; Hinz, R.; Haberer, T.; Jäkel, O.; Lauckner, K.; Pawelke, J.
no abstract
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Poster
IEEE Nuclear Science Symposium and Medical Imaging Conference, Albuquerque, New Mexico, 9-15 Nov, 1997
Book of Abstracts(1997)102 -
Contribution to proceedings
IEEE Nuclear Science Symposium and Medical Imaging Conference, Albuquerque, New Mexico, 9-15 Nov, 1997
Book of Abstracts(1997)102
Permalink: https://www.hzdr.de/publications/Publ-1040
Publ.-Id: 1040
ULIII Polarized XAFS Studies on Ba[UO2PO4]2.8H2O
Hennig, C.; Denecke, M. A.; Roßberg, A.; Zahn, G.; Reich, T.; Nitsche, H.
U LIII Polarized XAFS studies on Ba[UO2PO4]2·8H2O
C. Hennig 1, M. A. Denecke 1, A. Roßberg 1, G. Zahn 2,
T. Reich 1, H. Nitsche1
1 Forschungszentrum Rossendorf, Institut für Radiochemie,
PF 510119, D-01314 Dresden
2 Technical University of Dresden, Institute of Crystallography
and Solid State Physics, Zellescher Weg 16,
D-01062 Dresden
An experimental and theoretical study of the U LIII -edge polarization dependent XANES and EXAFS is presented for a single crystal of barium uranyl phosphate hydrate. Ba[UO2PO4]2·8H2O is built up by layers of [UO2]2+ and equatorial coordinated [PO4]3- tetrahedra. Layers are bridged by Ba2+, H+ and H3O+ cations giving an overall tetragonal (or nearly tetragonal) symmetry. The orientation of a crystal obtained by cleaving a larger crystal and used for the XAFS measurements was determined by x-ray diffraction. The layered structure of Ba[UO2PO4]2·8H2O exhibits preferred cleavage along {001} and parallel to {100}. Linear uranyl units are aligned parallel to [001]. {100} represents the least squares plane for the equatorial oxygen atoms. XAFS measurements were performed with the polarization vector aligned in the equatorial plane (parallel to [100] and [110]), as well as with the polarization vector oriented perpendicular to [010], with 90°, 60°, 45°, and 30° angles to [001].
Two different explanations of the resonance » 15 eV above the LIII -edge white-line maximum have been discussed. One explanation, based on pressure dependent measurements of UO3, attributed this feature to shake-up processes [1]. The other interpretation stems from ab initio multiple-scattering calculations using the FEFF program package. These calculations identify this feature as a multiple-scattering resonance associated with the axial U-O bonds in various uranium compounds [2], [3]. Our experimental investigations show that the relative intensity of this resonance increases if the polarization vector is aligned along the axial U-O bonds. This observation confirms the multiple-scattering assignment of this feature and is supported by our own theoretical FEFF calculations.
The U LIII -edge EXAFS show a strong polarization dependence, especially evident in the Fourier transforms at distances corresponding to uranyl axial oxygen atoms and equatorial atoms. This dependence strongly influences the effective coordination numbers, Ni, obtained in the data analysis.
The marked characteristics of such polarization-dependent XAFS spectra renders them useful as a unique indicator of uranyl orientation. For example, the specific binding sites and orientation of sorbed uranyl (actinyl) ions onto mineral surfaces can be determined with this method.
[1] Bertram, S., Kaindl, G., Jové, J., Pagès, M., Gal, J.: Phys.
Rev. B 52 (1989) 2680
[2] Hudson, E.A., Rehr, J.J., Buchner, J.J.: Phys. Rev. B 52
(1995) 13815
[3] Hudson, E.A., Allen, P.G., Terminello, L.J., Denecke, M.A.,
Reich, T.: Phys. Rev. B 54 (1996) 156
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Contribution to proceedings
Abstract für die Tagung der Deutschen Gesellschaft für Kristallographie 2.-5.3.1998 in Karlsruhe - Suppl. Z. Krist. 15, 156 (1998)
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Poster
Euroconference and NEA Workshop: Actinide-XAS-98, Grenoble, France, 04.-06.10.1998
Permalink: https://www.hzdr.de/publications/Publ-1039
Publ.-Id: 1039
Physically-based modeling of two-dimensional and three-dimensional implantation profiles: Influence of damage accumulation
Murthy, C. S.; Posselt, M.; Feudel, T.
The alteration of the shape of one-dimensional, two-dimensional (2D), and three-dimensional (3D) range distributions with growing dose as well as the extension of amorphous zones formed at high doses is studied for 15 keV BF2
+ and 30 keV P+ implantations into (100)Si using the dynamic binary collision code Crystal-TRIM. The range and damage profiles are calculated for the area 97.74 (parallel to [010]) × 97.74 (parallel to [001]) nm2 at the target surface irradiated by the ion beam and surrounded by impenetrable masks. The change of the shape of the 2D and 3D distributions in the lateral direction is less pronounced than in the depth direction. At low doses the lateral profile branches are determined by rechanneled particles, at high doses the enhanced dechanneling is the reason for the increased lateral straggling. The latter effect is responsible for the relatively large lateral extension of the amorphous zone beneath the masks. The simulated depth profiles of boron and phosphorus and the predicted thickness of the amorphous layer are in good agreement with experimental data.
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Journal of Vacuum Science and Technology B 16 (1998) 440
DOI: 10.1116/1.589828
Cited 2 times in Scopus -
Lecture (Conference)
Proc. 4th Int. Workshop Measurement, Characterization and Modeling of Ultra-Shallow Doping Profiles in Semiconductors, Res. Triangle Park, USA, April 1997
Permalink: https://www.hzdr.de/publications/Publ-1037
Publ.-Id: 1037
Structure Investigation of the Influence of the Irradiation Temperature on the Formation of Defects in Nuclear Pressure Vessel Steel A 533-B-1
Große, M.; Nitzsche, P.; Böhmert, J.; Hempel, A.; Brauer, G.; Haggag, F. M.
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Contribution to proceedings
Proceedings MRS 1996 Fall Meeting
Permalink: https://www.hzdr.de/publications/Publ-1036
Publ.-Id: 1036
Präparation und In-Vivo-Testung von Melanom-affinen '3+1' (99mTc)-Oxotechnetium(V)-Gemischt-Ligandkomplexen
Friebe, M.; Spies, H.; Johannsen, B.; Mohammed, A.; Eisenhut, M.
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Lecture (Conference)
DGN-Tagung, 36. Internationale Jahrestagung, Leipzig, 01.-04. April 1998 -
Abstract in refereed journal
Nuklearmedizin 37 (1998) A49
Permalink: https://www.hzdr.de/publications/Publ-1035
Publ.-Id: 1035
Rezeptoraffine Oxorhenium(V)-Komplexe als Inhibitoren der Monoaminoxidase im Rattenhirn
Matys, S.; Brust, P.; Scheunemann, M.; Pietzsch, H.-J.; Johannsen, B.
In früheren Untersuchungen haben wir nachgewiesen, dass Oxorhenium(V)-Komplexe mit Ketanserin-, Cisaprid- und MDL72832-ähnlicher Struktur hohe Affinität zu Serotoninrezeptoren des Gehirns aufweisen, womit die analogen 99mTc-Verbindungen als potentielle Radiopharmaka von Interesse sind. Ihre Struktur ließ auch inhibitorische Wirkung auf die Serotonin abbauende Monoaminoxidase (MAO) vermuten. In Untersuchungen an Rattenhirnhomogenaten mit 1mM Tryptamin als Substrat beider Isoenzyme MAO A und MAO B, bzw. 1 mM Phenylethylamin als spezifisches Substrat für MAO B hemmt die Mehrheit der untersuchten Komplexe mit IC50 Werten zwischen 10-4 und 10-6 M das Enzym. Die höchste Affinität besitzt der abgebildete Komplex mit IC50=7*10-7±2 M.
Die räumliche Anordnung des protonierbaren Stickstoffs im Molekül ist dabei kritisch. Die Ergebnisse zeigen, daß bei der Bewertung von Radiotracern für das serotonerge System potentielle Wechselwirkungen mit der MAO berücksichtigt werden müssen.
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Poster
36. Intern. Jahrestagung DGN, Leipzig, 01.-04.04.1998 -
Abstract in refereed journal
Nuklearmedizin 37 (1998) A51
Permalink: https://www.hzdr.de/publications/Publ-1034
Publ.-Id: 1034
Rheniumkomplexe von Steroidalen Estrogenen, Androgenen und Progestinen
Wüst, F.; Berger, R.; Katzenellenbogen, J. A.; Alberto, R.; Schubiger, P. A.; Spies, H.; Johannsen, B.
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Lecture (Conference)
36. Intern. Jahrestagung der DGN, Leipzig, 01.-04. April, 1998 -
Abstract in refereed journal
Nuklearmedizin 37 (1998) A45
Permalink: https://www.hzdr.de/publications/Publ-1033
Publ.-Id: 1033
Beeinflussung der99mTc-MIBI- und [18F]FDG-Aufnahme durch Inhibitoren des P-Glycoproteins
Bergmann, R.; Brust, P.; Johannsen, B.
Das P-Glycoprotein (Pgp) ist ein energieabhängiges Efflux-Transportsystem für ein breites Pharmaka-Spektrum, welches in bestimmten Tumoren, aber auch in normalen Geweben, z. B. den Endothelzellen des Gehirns exprimiert wird. Die Pgp-Bewertung in Tumoren mit lipophilen Kationen (99mTc-MIBI, 99mTc-Tetrafosmin) wird durch verschiedene biochemische Veränderungen (z. B. des Energiestoffwechsels) erschwert. In Multitracerexperimenten an Hirnendothelzellen untersuchten wir die Veränderungen im Membranpotential (99mTc-MIBI, 99mTc-Tetrafosmin), des Glukoseumsatzes ([18F]FDG) und der Pgp-Aktivität ([3H]Vinblastin) unter dem Einfluß verschiedener Pgp-Inhibitoren (u. a. Verapamil, Vinblastin,Valinomycin). Die Zellaufnahme der Pgp-Substrate ([3H]Vinblastin, 99mTc-MIBI, 99mTc-Tetrafosmin) korrelliert unter Kontrollbedingungen mit dem Glucosemetabolismus ([18F]FDG). Bei Hemmung des Pgp zeigte sich allerdings in den meisten Fällen eine Verminderung der Akkumulation von FDG. Das Ionophor Valinonycin löst dagegen einen dramatischen Anstieg des Glucoseumsatzes aus, gleichzeitig ist die MIBI oder Tetrafosmin-Aufnahme verringert obwohl die [3H]Vinblasin-Akkumulation unverändert bleibt. Das zeigt, daß bei der Untersuchung von Pgp-Transportprozessen Sekundäreffekte auftreten können (hier Veränderungen des Energiestoffwechsels), die bei der Interpretation der Daten zu berücksichtigen sind.
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Lecture (Conference)
36. Intern. Jahrestagung DGN, Leipzig, 01.-04.04.1998 -
Abstract in refereed journal
Nuklearmedizin 37 (1998) A17
Permalink: https://www.hzdr.de/publications/Publ-1032
Publ.-Id: 1032
Thermochromatography of Heavy Actinides - Adsorption of No-259 on Ti, V, Nb, Ta and Mo
Taut, S.; Hübener, S.; Eichler, B.; Türler, A.; Gäggeler, H. W.; Timokhin, S. N.; Zvara, I.
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Journal of Alloys and Compounds 271-273 (1998) 316-321
DOI: 10.1016/S0925-8388(98)00079-6
Cited 3 times in Scopus - J. Less-Common Met. 271-273, 316 (1998)
Permalink: https://www.hzdr.de/publications/Publ-1030
Publ.-Id: 1030
Decay Study of Hot Nuclei below the Multifragmentation Threshold with the FOBOS Detector at Dubna
Herbach, C.-M.; Ortlepp, H.-G.; Wagner, W.
Abstract
The first series of experiments at the FOBOS detector, using beams of the U-400M cyclotron of the Flerov Laboratory of Nuclear Reactions, was devoted to few-fragment decays of equilibrated systems. To exclude deep inelastic collisions or quasifission as sources of massive fragments, hot heavy nuclei were produced in the very asymmetric reactions 7Li (43 AMeV) + 232Th, 14N (34 AMeV) + 197Au, and 14N (53 AMeV) + 197Au, 232Th. Two- and three-fragment events were analysed on the base of masses and velocity vectors measured independently for each fragment. The events were sorted into excitation energy bins according to the linear momentum transfer following the massive transfer approach. Binary events were treated as fission. Fragment mass distributions as well as total kinetic energies were studied for an excitation energy range of 100 - 500 MeV. A new TKE parametrisation is proposed extending the Viola systematics to large mass asymmetries. With rising excitation energy the mass dispersion develops unexpectedly. Two new effects have been fourid and are discussed as consquences of the cooling down during the slow fission process at moderate E*, and of a strong decrease of the fission time at large E*. Ternary events were analysed by comparing measured velocity correlations with results of Coulomb trajectory simulations. If one fragment has intermediate mass (A = 10...30), two components in the relative velocities and the Z/A ratios confirm a sequential and a neck mechanism. For events with three fragments of comperable size neither the assumption of two sequential independent fission acts nor a nlultifragnlentaion-like scenario can reproduce the data. Agreement is achieved if these three-fragment decays are characterized by a collinear intermediate state followed by two scissions separated by no more than 280 fm/c, a very short time scale compared with usual saddle-to-scission intervals.
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Forschungszentrum Rossendorf; FZR-198
ISSN: 1436-3976 -
Other report
Konferenzbeitrag HIPH '97
Downloads
Permalink: https://www.hzdr.de/publications/Publ-1029
Publ.-Id: 1029
Metal Plasma Immersion Ion Implantation and Deposition (MPIIID): Chromium on Magnesium
Brückner, J.; Günzel, R.; Richter, E.; Möller, W.
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Poster
Konferenz SMMIB 97, Gatlinburg, TE, USA, Sept. 1997 -
Surface and Coatings Technology 103-104 (1998) 227-230
DOI: 10.1016/S0257-8972(98)00399-5
Cited 25 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1028
Publ.-Id: 1028
Complexation of Uranium(VI) with the Main Components of Mine-Wood Degradation. Part 1. Complexation with Protocatehuic Acid, Vanillic Acid and Vanillin
Baraniak, L.; Schmidt, M.; Bernhard, G.; Nitsche, H.
To consider the process of mine wood degradation and its concequences on the contaminant migration via aquatic path in risk assessments, e.g. for uranium mine restoration in the southern region of Saxony (Germany), the complexation of U(VI) with 3,4-dihydroxybenzoic acid (proto-catechuic acid), 4-hydroxy-3-methoxy-cinnamic acid (ferulic acid), 4-hydroxy-3-methoxybenzoic acid (vanillic acid) and 4-hydroxy-3-methoxybenzaldehyde (vanillin) was studied by potentiometric pH titration in carbonate-free solutions of 0.1 M NaClO4. These four complexants are reasonably stable monomeric intermediates in the microbial or hydrothermally driven spruce-wood lignin degradation and therefore play a role in natural water chemistry.
The evaluation of the pH titration curves was carried out with the classical theory of stepwise complex formation, analyzing Bjerrums formation function [1] and by non-linear fitting of the pH titration curve with Sayces multi-equilibria program "SCOGS" [2], considering hydrolysis and mixed-ligand complexation.
In the case of protocatechuic acid, a series of very stable (1:1) to (1:3) complexes are formed (log ß: 14.8/25.9/33.2). The constants calculated by Bjerrums formation function are in full agreement with the values of the SCOGS curve fitting, i.e. U(VI) hydrolysis is surpressed in the presence of this ligand. The complexes with ferulic acid and vanillic acid have a much lower stability: log ß11 values are to 6.88 and 7.16, respectively. In the case of ferulic acid, the assumption of the acidic species [UO2H(fer)]+ with log ß111 =11.9 improves the pH curve fit. Vanillin as complexant leads to pH curves that can be best fitted with the species [UO2(van)]+ and [UO2(van)2(OH)2]2- with log ß values of 4.47 and -3.95, respectively.
Using these data speciation calculations for some calcite-rich mine waters show that the strong U(VI)-carbonato complexes predominate. Under certain conditions only protocatechuic acid complexes can be formed.
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Poster
6th International Conference on Chemistry and Migration Behaviour of Actinides and Fission Products in the Geosphere: MIGRATION '97, Sendai, Japan, October 26-31, 1997
Permalink: https://www.hzdr.de/publications/Publ-1027
Publ.-Id: 1027
Characterization of the Redox Behaviour of Spruce-Wood Lignin and Humic Acid
Mack, B.; Abraham, A.; Baraniak, L.; Bernhard, G.; Nitsche, H.
The redox behaviour of spruce lignin and humic acid was characterized by their redox potential and redox capacity. Such polyelectrolytes are formed in natural degradation processes including wood decomposition. They influence the redox situation in water of flooded uranium mines.
The first approach to the standard potential using a platinum electrode in combination with a silver-siver chloride electrode (3 M KCl) in a cell with liquid junction [1] was done in two ways: (1) by direct redox potential measurements [2] and (2) by redox titration with potassium hexacyanoferrate(III) [3], both in dependence on the pH. The redox potential of spruce lignin at pH 0 determined in that way was found to be 580±20 mV. That represents a rough E0 which can be arranged in the series of redox couples with decreasing E0. The reduction capacity determined from the titration at pH 9 amounts to 15±0.5 meq/g. Iron(III) in non-complexing solution (0.1 M KCl) was completely reduced by lignin with a maximum capacity of 6.5±0.8 meq/g in the pH range 2 to 2.5. Humic acids of different origin are characterized in the same way.
In addition, the iron(III) reduction by lignin and humic acid was examined in the pH range 3 to 5 by sqare-wave voltammetric analysis after a four weeks equilibration under inert gas at 25 °C. The iron(III) waves at -1.40 V and -1.60 V disappeared and the typical iron(II) signal was found at -1.33 V (all potentials were measured vs. Ag/AgCl, 3 M KCl). Changing the iron(III)-lignin ratio at pH 4.7±0.2 the maximum iron(III) quantity that can be reduced by a given lignin amount could be determined to 4.0 meq/g. At higher ratios the wave of the unreduced iron(III) was detected at -1.6 V (pH 4). At ratios below 4 meq/g iron(III) is quantitatively reduced and there is a linear relationship between the introduced iron(III) concentration and the intensity of the found iron(II) signal.
The analytical proof of the formed iron(II) was carried out by spectrophotometric determination with o-phenantroline. This sensitive method with a detection limit of 0.01 ppm iron(II) was adapted in such a way that iron(II) could be determined in the presence of iron(III).
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Poster
13th Radiochemical Conference, Marianske Lazne - Jachymov, Czech Republic, April 20.-24.04.1998
Permalink: https://www.hzdr.de/publications/Publ-1026
Publ.-Id: 1026
Simultaneous Measurement of 18F-FDOPA Metabolism and Cerebral Blood Flow in Newborn Piglets
Brust, P.; Bauer, R.; Walter, B.; Bergmann, R.; Füchtner, F.; Vorwieger, G.; Steinbach, J.; Johannsen, B.; Zwiener, U.
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Int. J. Devl. Neuroscience, Vol. 16, No. 5, pp 353-364, 1998
DOI: 10.1016/S0736-5748(98)00017-3
Cited 13 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1025
Publ.-Id: 1025
A Method for the Intrinsic Calibration of CsI(Tl) Detectors
Kamanin, D. V.; Wagner, W.; Ortlepp, H.-G.
Abstract
A method for the intrinsic energy calibration of photomultiplier-coupled CsI(Tl) detectors is described. A simple empirical model of the scintillation light pulse-shape of CsI(Tl) crystals for light charged particles has been applied to simulate the particle identification matrix as it follows from the pulse-shape analysis method. The calibration procedure for the large-area CsI(Tl) detectors of the scintillator shell of the 4 π - array FOBOS for ions with Z < 4 at energies below 100 AMeV is based on the energies of the particle punch-through points.
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Forschungszentrum Rossendorf; FZR-197
ISSN: 1436-3976 -
Nuclear Instruments and Methods in Physics Research A 413 (1998) 127-137
DOI: 10.1016/S0168-9002(98)00467-7
Cited 5 times in Scopus
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Permalink: https://www.hzdr.de/publications/Publ-1023
Publ.-Id: 1023
RBS and Channeling Analysis of Cobalt Disilicide Layers Produced by Focused Ion Beam Implantation
Teichert, J.; Voelskow, M.; Bischoff, L.; Hausmann, S.
Cobalt disilicide layers were formed by ion beam synthesis using 35 keV Co+ focused ion beam (FIB) implantation into silicon. A strong influence of the pixel dwell time on the layer formation was found. Only for short pixel dwell-times (about 1µs) closed layers with sufficient quality for device application could be formed. To understand the dwell-time effect the as-implanted samples were examined by Rutherford backscattering (RBS) and channeling analysis. A method is presented which allows quantitative measurements of samples where the implanted areas are smaller than the diameter of the RBS beam. Evidence has been obtained that the silicon crystal damage is less for short dwell-times.
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Vacuum, Volume 51, Number 2, Pages 261-266, 1998
DOI: 10.1016/S0042-207X(98)00171-7
Cited 6 times in Scopus -
Lecture (Conference)
10th Int. School on Vacuum, Electron and Ion Technologies, Varna, Bulgaria, Sept. 22 - 27, 1997
Permalink: https://www.hzdr.de/publications/Publ-1022
Publ.-Id: 1022
Elastic Proton-Deuteron Backward Scattering: Relativistic Effets and Polarization Observables
Kaptari, L. P.; Kämpfer, B.; Dorkin, S. M.; Semikh, S. S.
Abstract
The elastic proton-deuteron backward reaction is analyzed within a covariant approach based on the Bethe-Salpeter equation with realistic meson-exchange interaction. Lorentz boost and other relativistic effects in the cross section and spin correlation observables, like tensor analyzing power and polarization transfer etc., are investigated in explicit form. Results of numerical calculations for a compbte set of polarization observables are presented.
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Forschungszentrum Rossendorf; FZR-194
ISSN: 1436-3976 -
Physical Review C Vol. 57 (1998) 1097-1111
DOI: 10.1103/PhysRevC.57.1097
Cited 27 times in Scopus
Downloads
Permalink: https://www.hzdr.de/publications/Publ-1021
Publ.-Id: 1021
Verification of the Code DYN3D/R with the Help of International Benchmarks
Grundmann, U.; Rohde, U.
Different benchmarks for reactors with quadratic fuel assemblies were calculated with the code DYN3D/R. In this report comparisons with the results of the reference solutions are carried out. The results of DYN3D/R and the reference calculation for the eigenvalue keff and the power distribution are shown for the steady-state 3-dimensional IAEA-Benchmark. The results of NEACRP-Benchmarks on control rod ejections in a standard PWR were compared with the reference solutions published by the NEA Data Bank. For assessing the accuracy of DYN3D/R results in comparison to other codes the deviations to the reference solutions are considered. Detailed comparisons with the published reference solutions of the NEA-NSC Benchmarks on uncontrolled withdrawal of control rods are made. The influence of the axial nodalization is also investigated. All in all, a good agreement of the DYN3D/R results with the reference solutions can be seen for the considered benchmark problems.
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Forschungszentrum Rossendorf; FZR-195 October 1997
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-1020
Publ.-Id: 1020
Entwicklung von theoretischen Schwingungsmodellen für WWER-Reaktoren auf der Grundlage der Finite-Elemente-Methode
Altstadt, E.; Weiß, F.-P.; Werner, M.; Bulavin, V.; Pavelko, V.; Gutsev, D.; Anikin, G.; Usanov, A.; Dodonov, V.
In diesem Abschlußbericht wird ein Fördervorhaben beschrieben, welches auf die Unterstützung von 6 russischen Wissenschaftlern aus drei unterschiedlichen Institutionen abzielte. Ihre Arbeiten zur Anlagendiagnostik / Schadensfrüherkennung dienen der Erhöhung der Sicherheit von WWER-Reaktoren.
Das Vorhaben leistet einen Beitrag zur verbesserten Beurteilung der mechanischen Integrität von Reaktoren der russischen WWER-440 und WWER-1000 Baureihe, insbesondere zur empfindlichen Früherkennung und Lokalisation mechanischer Schädigungen an Reaktorkomponenten mit Hilfe schwingungsdiagnostischer Methoden. Zu diesem Zweck wurde das Finite-Element-Modell zur Simulation des mechanischen Schwingungsverhaltens aller Primärkreiskomponenten eines WWER-1000 erstellt. Dafür wurde das Programmpaket ANSYS® genutzt.
Das Berechnungsmodell zum WWER-440 wurde mit neueren Ergebnissen experimenteller Schwingungsuntersuchungen weiter justiert. Das Modell kann in der Hauptsache genutzt werden, um zu klären, wie sich unterstellte mechanische Defekte von Reaktoreinbauten auf die Schwingungen der Gesamtanlage auswirken. Diese Schadenssimulation ist besonders geeignet, empfindliche Meßpositionen für die on-line Überwachung zu finden und physikalisch fundierte Grenzwerte zu definieren.
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Forschungszentrum Rossendorf; FZR-196 Oktober 1997
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-1019
Publ.-Id: 1019
Ellipsometric Investigation of Damage Distribution in Low Energy Boron Implantation of Silicon
Fukarek, W.; Möller, W.; Hatzopoulos, N.; Armour, D. G.; van den Berg, J. A.
As the scaling of silicon devices to 100 nm channel length requires the formation of ultra-shallow (< 60 nm) junctions, high depth resolution analytical techniques become necessary for the characterization of the dopant and damage distributions. In situ single wavelength Ellipsometric
Etch Depth Profiling (EEDP) and non-destructive Variable Angle of incidence Spectroscopic Ellipsometry (VASE) have been used to obtain accurate and quantitative information on the depth profiles of radiation damage produced by low energy, room temperature ion implantation of B+ into Si.
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Nuclear Instruments and Methods in Physics Research B 127/128 (1997) 879-883
DOI: 10.1016/S0168-583X(97)00024-4
Cited 21 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1018
Publ.-Id: 1018
Verhalten des Radiums im Flutungsprozeß des Uranbergwerks Königstein
Baraniak, L.; Thieme, M.; Funke, H.; Bernhard, G.; Nitsche, H.
The interaction of radium with characteristic sediments of the upper Saxon Elbe river valley was investigated with the
aim to provide key data for transport modelling within the framework of mining site restoration. Adsorption
measurements therefore were carried out on site-specific sediments (different kinds of sandstone, claystone and lime
marl) using (1) acidic mine water coming from sulfuric acid residues of the former in-situ leaching process, (2)
groundwater that is inflowing into the mine and (3) mixtures of both which simulates certain stages of the mine flooding process. The distribution ratios were determined by batch experiments using an eight-week equilibration at aquifer temperature (14 °C). Radium adsorption from acidic mine water onto different kinds of sandstone is characterized by high distribution ratios (3400 mL/g). When contacted with groundwater, the sorption is decreased more than 20-fold (60-180 mL/g). For claystone and lime marl the distribution ratios amount to 130 and 480 mL/g, respectively, and they are nearly constant in the mine flooding process. The main adsorption mechanisms on the leached sandstone and the clayey sediments were identified as coprecipitation and ion exchange, respectively. The long-term migration behaviour in the aquifers of the south-east Saxon Elbe basin was calculated on the basis of Hadermanns' equation, considering retardation, dispersion and radioactive decay.
- Wissenschaftliche Zeitschrift der TU-Dresden 46 (1997) Heft 6, S. 90-94
Permalink: https://www.hzdr.de/publications/Publ-1016
Publ.-Id: 1016
Interaction of Uranium(VI) with Arsenate in Aqueous Solution Studied by Time-Resolved Laser-Induced Fluorescence Spectroscopy (TRLFS)
Rutsch, M.; Geipel, G.; Bernhard, G.; Nitsche, H.
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Poster
13th Radiochemical Conference, Marianske Lasne-Jachymov, Czech Republik, 20.-24.04.1998 -
Radiochimica Acta 86(1999), 135-141
DOI: 10.1524/ract.1999.86.34.135
Cited 37 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1014
Publ.-Id: 1014
Methods for Colloid Characterization in Environmental Waters Rich in Humic Substances
Zänker, H.; Richter, W.; Hüttig, G.; Schmeide, K.; Nitsche, H.
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Poster
13th Radiochemical Conference, Marianske Lazne, 19-24.4.1998
Permalink: https://www.hzdr.de/publications/Publ-1013
Publ.-Id: 1013
Fine Structure of the E1 Response in 140Ce Below the Particle Threshold*
Herzberg, R.-D.; von Brentano, P.; Eberth, J.; Enders, J.; Fischer, R.; Huxel, N.; Klemme, T.; von Neumann-Cosel, P.; Nicolay, N.; Pietralla, N.; Ponomarev, V. Y.; Reif, J.; Richter, A.; Schlegel, C.; Schwengner, R.; Skoda, S.; Thomas, H. G.; Wiedenhöver, I.; Winter, G.; Zilges, A.
The E1 response of the semi-magic nucleus 140Ce below the particle
threshold was measured in a (gamma, gamma') experiment utilizing the new
Euroball Cluster detector at the S-DALINAC. While the energy averaged data
are in good agreement with the tagged photon results, here they are resolved
for the first time into 54 individual transitions. A quasiparticle-phonon
model calculation including up to three-phonon configurations compares
well to the extracted strength distribution. The interference between one-
and two-phonon contributions is essential for a quantitative reproduction.
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Physics Letters B 390 (1997) 49-54
DOI: 10.1016/S0370-2693(96)01374-3
Cited 91 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1011
Publ.-Id: 1011
Tilted Rotation of Weakly Deformed and Triaxial Nuclei
Frauendorf, S.
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Zeitschrift für Physik A 358, 163-167 (1997)
DOI: 10.1007/s002180050295
Permalink: https://www.hzdr.de/publications/Publ-1010
Publ.-Id: 1010
Dipole excitations in 122Te, 126Te and 130Te
Schwengner, R.; Schauer, W.; Winter, G.; von Brentano, P.; Eberth, J.; Enders, J.; von Egidy, T.; Grinberg, M.; Herzberg, R.-D.; Huxel, N.; Käubler, L.; von Neumann-Cosel, P.; Nicolay, N.; Ott, J.; Pietralla, N.; Prade, H.; Raman, S.; Reif, J.; Richter, A.; Schlegel, C.; Schnare, H.; Servene, T.; Skoda, S.; Stoyanov, C.; Thomas, H. G.; Wiedenhöver, I.; Zilges, A.
Excited states of the nuclei 122Te, 126Te and 130Te
were populated via the (gamma,gamma') reaction at endpoint energies of
the bremsstrahlung between 4.5 and 5.5 MeV. Gamma rays were detected with
a EUROBALL-CLUSTER detector and a single detector. In all nuclei several
dipole transitions were identified at energies around 3 MeV. The lowest
corresponding J = 1 states are interpreted as two-phonon excitations. Quasiparticle-phonon-model
calculations predict one 1- state arising from the coupling
of the first quadrupole and the first octupole phonon and one 1+
state arising from the coupling of the first and the isovector second quadrupole
phonon at about 3 MeV. The calculated transition strengths are compatible
with experimental one.
- Zeitschrift für Physik A 358, H.2, 197-198 (1997)
Permalink: https://www.hzdr.de/publications/Publ-1008
Publ.-Id: 1008
Particle-hole Induced Intruder Bands in117Sb and 119Sb
Lafosse, D. R.; Fossan, D. B.; Hughes, J. R.; Liang, Y.; Schnare, H.; Vaska, P.; Waring, M. P.; Zhang, J. Y.
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Physical Review C Volume 56, Number 2, 760-771
DOI: 10.1103/PhysRevC.56.760
Cited 32 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1007
Publ.-Id: 1007
Fragmentation of the Yrast Band in 186Os at Ipi=18+ and Disappearance of the Collective Minimum
Balabanski, D. L.; Hristov, D. H.; Lieder, R. M.; Rzaca-Urban, T.; Gast, W.; Hebbinghaus, G.; Krämer-Flecken, A.; Schnare, H.; Urban, W.; Wyss, R.
- Zeitschrift für Physik A 356, 393-397 (1997)
Permalink: https://www.hzdr.de/publications/Publ-1006
Publ.-Id: 1006
The application of PET to quality assurance of heavy-ion tumour therapy.
Enghardt, W.; Debus, J.; Haberer, T.; Hasch, B.-G.; Hinz, R.; Jäkel, O.; Krämer, M.; Lauckner, K.; Pawelke, J.
At the new heavy ion tumor therapy facility of the Gesellschaft für Schwerionenforschung at Darmstadt positron emission tomography (PET) has been implemented for in-beam and in-situ therapy control, i.e. during the tumor irradiation. The components necessary for this dedicated PET-imaging and their integration into the framework of therapy planning and quality assurance of heavy ion cancer treatments are presented. Results of the first application of this PET-method to patient treatments are reported.
Keywords: heavy-ion therapy; positron emission tomography; treatment planning; quality assurance
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Strahlentherapie und Onkologie, Vol. 175, Suppl. II (1999) 33-36
DOI: 10.1007/BF03038884
Cited 48 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1005
Publ.-Id: 1005
Solution of the 4th AER Dynamic Benchmark by Use of the Code DYN3D with a Particle-in-Cell Method for the Description of Boron Transport
Rohde, U.; Lucas, D.
The results of the 4th AER dynamic benchmark obtained by the use of the code DYN3D in the Research Centre Rossendorf are presented. The benchmark comprises the modeling of a boron dilution transient caused by switching on the first main coolant pump of a loop containing a plug of partially undiluted water. Therefore, the course of the transient is significantly affected by correct modeling of the boron transport. The results of studies on the influence of numerical diffusion during boron transport are presented. Consequently, a new numerical model based on the particleincell method has been developed and implemented into DYN3D. The basic features of this model are described. It allows the complete suppression of numerical diffusion and to take into account the effect of boron enrichment in the liquid water phase in the case of boiling in a simple manner. Another important feature of the benchmark task was that each participant had to use his own macroscopic cross section library. In our analysis the MAGRU library for VVER440 was used. A few reactorphysical key parameters had been given in the benchmark definition for optional adoptation of the cross section data. The presented analysis was carried out with a minimum amount of adoptations. Finally, only the static supercriticality of the boron dilution was given an the Doppler feedback was adopted. Some interesting thermohydraulic effects are discussed, which can be used for a deeper comparative analysis of the thermohydraulics models of the codes. Due to the low mass flow rate and high heat flux densities occuring, vapour generation during the transient is significantly affected by subcooled boiling under thermodynamic nonequlibrium conditions.
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Lecture (Conference)
7th Symposium of Atomic Energy Research, Hörnitz, 23. - 26. 09. 1997 -
Contribution to proceedings
Proceedings of the 7th Symposium of Atomic Energy Research, p. 387, Hörnitz, 23. - 26. 09. 1997
Permalink: https://www.hzdr.de/publications/Publ-1004
Publ.-Id: 1004
Strong Blue and Violet Photo- and Electroluminescence from Germanium- and Silicon-Implanted Silicon Dioxide Layers
Rebohle, L.; von Borany, J.; Yankov, R. A.; Skorupa, W.; Tyschenko, I. E.; Fröb, H.; Leo, K.
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Applied Physics Letters, Vol. 71, Nr. 19, S. 2809-2811
DOI: 10.1002/(SICI)1521-396X(199801)165:1<31::AID-PSSA31>3.0.CO;2-Y
Cited 14 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1002
Publ.-Id: 1002
MARS: A Start Detector System for the Cosy Time-of-Flight Spectrometer TOF
Michel, P.; Möller, K.; Naumann, B.; Naumann, L.; Schamlott, A.; Schmidt, G.; Schülke, A.
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Nuclear Instruments and Methods in Physics Research A 408 (1998) 453-467
DOI: 10.1016/S0168-9002(98)00220-4
Cited 4 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-1001
Publ.-Id: 1001
11C-Labelling of Heterocyclic Aromatic Compounds in Ring Positions: Synthesis of 2-11C Indole
Zessin, J.; Steinbach, J.
- Journal of Labelled Compounds and Radiopharmaceuticals XLI, 669-676 (1998)
Permalink: https://www.hzdr.de/publications/Publ-1000
Publ.-Id: 1000
Synthesis of Oxorhenium(V) Complexes Derived from 7-alpha-Functionalized Testosterone: First Rhenium-Containing Testosterone Derivatives
Wüst, F.; Scheller, D.; Spies, H.; Johannsen, B.
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Eur. J. Inorg. Chem. 1998, 789-793
DOI: 10.1002/(SICI)1099-0682(199806)1998:6<789::AID-EJIC789>3.0.CO;2-Z
Cited 17 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-999
Publ.-Id: 999
In-beam PET imaging for the control of heavy-ion tumour therapy.
Pawelke, J.; Enghardt, W.; Haberer, T.; Hasch, B.-G.; Hinz, R.; Krämer, M.; Lauckner, K.; Sobiella, M.
A method for the in-situ control of the heavy-ion tumour therapy by means of positron emission tomography is introduced. This method is founded on the measurement of the dynamic spatial distributions of beta+-emitters generated by nuclear fragmentation during the irradiation and their relation to the dose. In order to study this relationship and to derive the dose distribution from the measured beta+-activity distribution, a framework of model calculations is used. Results of phantom experiments with 12C ion beams will be presented, demonstrating good agreement between experiment and calculation as well as the possibilities and limits of the PET-technique for treatment plan verification and beam monitoring.
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IEEE Transactions on Nuclear Science, Vol. 44, No. 4 (1997) 1492-1498
DOI: 10.1109/23.632694
Cited 83 times in Scopus -
Lecture (Conference)
IEEE Nuclear Science Symposium, 2-9 Nov, 1996, Anaheim, California, USA
Conference Record, Vol. 2 (1996) 1099-1103 -
Contribution to proceedings
IEEE Nuclear Science Symposium, 2-9 Nov, 1996, Anaheim, California, USA
Conference Record, Vol. 2 (1996) 1099-1103
Permalink: https://www.hzdr.de/publications/Publ-998
Publ.-Id: 998
Tilted Rotation and Backbending in an Odd-Proton Nucleus
Pearson, C. J.; Walker, P. M.; Purry, C. S.; Dracoulis, G. D.; Bayer, S.; Byrne, A. P.; Kibedi, T.; Kondev, F. G.; Shizuma, T.; Bark, R. A.; Sletten, G.; Frauendorf, S.
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Physical Review Letters, Volume 79, Number 4
DOI: 10.1103/PhysRevLett.79.605
Cited 33 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-997
Publ.-Id: 997
Fission of Metal Clusters
Näher, U.; Bjornholm, S.; Frauendorf, S.; Garcias, F.; Guet, C.
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Physics Reports 285 (1997) 245-320
DOI: 10.1016/S0370-1573(96)00040-3
Cited 264 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-996
Publ.-Id: 996
Identification of Excited States in Doubly Odd 110Sb: Smooth Band Termination
Lane, G. J.; Fossan, D. B.; Thorslund, I.; Vaska, P.; Allatt, R. G.; Paul, E. S.; Käubler, L.; Schnare, H.; Hibbert, I. M.; O'Brien, N.; Wadsworth, R.; Andrejtscheff, W.; de Graaf, J.; Simpson, J.; Lee, I. Y.; Macchiavelli, A. O.; Blumenthal, D. J.; Davids, C. N.; Lister, C. J.; Seweryniak, D.; Afanasjev, A. V.; Ragnarsson, I.
Excited states in 110Sb have been identified for the first time
in a series of gamma-spectroscopy experiments using both thin and backed
targets, including neutron-fold and recoil-mass measurements to provide
unambiguous channel identification. The three decoupled intruder bands
observed in 110Sb are based upon configurations involving 2p-2h
excitations across the Z=50 shell gap and show the features of smooth band
termination. The yrast intruder band, which has been connected to the low-spin
levels, is tentatively identified up to its predicted termination at IPi=45+.
Excellent agreement with configuration-dependent cranked Nilsson-Strutinsky
calculations is obtained for the high-spin states near termination.
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Physical Review C, Nuclear Physics, 3rd Series, Volume 55, Number 5
DOI: 10.1103/PhysRevC.55.R2127
Cited 34 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-995
Publ.-Id: 995
Influence of the Ion Irradiation on the Properties of ß-FeSi2 Layers Prepared by Ion Beam Assisted Deposition
Barradas, N.; Panknin, D.; Wieser, E.; Schmidt, B.; Betzl, M.; Mücklich, A.; Skorupa, W.
ß-FeSi2 was produced by ion beam assisted deposition
(IBAD). The influence of the deposition parameters on the structure was
studied by Rutherford backscattering, X-ray diffraction, cross section
transmission electron microscopy, and scanning electron microscopy. The
samples grow in a columnar way with pin-holes and their surface is rough.
A soft IBAD process with low Ar energy (EAr = 200 eV) and low Ar ion to
Fe atom ratio (IAr/AFe = 0.16) improves the layer structure in comparison
to samples prepared without Ar irradiation. Less pin-holes are formed,
and the roughness shows a minimum. The roughness increases for larger EAr
and larger IAr/AFe. All samples are polycrystalline but with a pronounced
texture. The preferential orientation is also enhanced by the IBAD process.
The electrical properties of the layers were characterized by Hall effect
measurements and measurements of the I-V characteristics of simple diode
structures. The results are discussed in relation with the influence of
the ion beam.
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Nuclear Instruments and Methods in Physics Research B 127/128(1997) 316-320
DOI: 10.1016/S0168-583X(96)00947-0
Cited 4 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-994
Publ.-Id: 994
Pion Production in Mass-Symmetric Heavy Ion Collisions at 0.8-1.8 AGeV
Müntz, C.; Baltes, P.; Oeschler, H.; Sartorius, C.; Sturm, C.; Wagner, A.; Bormann, C.; Brill, D.; Shin, Y.; Stein, J.; Ströbele, H.; Ahner, W.; Barth, R.; Cieslak, M.; Debowski, M.; Grosse, E.; Henning, W.; Koczon, P.; Mang, M.; Miskowiec, D.; Schicker, R.; Senger, P.; Kohlmeyer, B.; Pöppl, H.; Pühlhofer, F.; Speer, J.; Völkel, K.; Walus, W.
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Zeitschrift für Physik A 357, 399-409 (1997)
DOI: 10.1007/s002180050259
Permalink: https://www.hzdr.de/publications/Publ-993
Publ.-Id: 993
Jahresbericht 1995/1996 Abteilung Kommunikation und Datenverarbeitung
Fülle, R.
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Forschungszentrum Rossendorf; FZR-187
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-992
Publ.-Id: 992
In-situ Investigation of Ion Drift Processes in Glass During Anodic Bonding
Schmidt, B.; Nitzsche, P.; Lange, K.; Grigull, S.; Kreißig, U.; Thomas, B.; Herzog, K.
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Lecture (Conference)
EUROSENSORS XI, The 11th European Conference on Solid-State Transducers , Warzaw, Poland, Sept. 21-24, 1997 -
Sensors and Actuators A 67 (1998) 191-198
DOI: 10.1016/S0924-4247(97)01768-8
Cited 43 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-991
Publ.-Id: 991
Elektroenergieerzeugung aus erneuerbaren Energiequellen in Sachsen
Hackstein, G.; Riedel, J.; Rindelhardt, U.; Schwanitz, M.
Im Bericht werden die Potentiale zur Elektroenergieerzeugung aus verschiedenen erneuerbaren Energiequellen in Sachsen zusammengestellt. Dabei werden natürliche Potentiale und - wo möglich - technische Potentiale sowie wirtschaftliche Potentiale unterschieden. Das ermittelte technische Potential (ohne Biomasse) entspricht etwa einer Elektroenergieproduktion von 7400 GWh jährlich. Davon entfallen etwa 2/3 auf die Windenergie und der Rest zu gleichen Teilen auf die Wasserkraft und die Photovoltaik.
Die Erschließung der Potentiale seit 1990 wird im Einzelnen dargestellt. Neben der seit langem genutzten Wasserkraft entwickelt sich insbesondere die Windenergie sehr dynamisch. Die Windenergie wird noch 1997 die Wasserkraft als bedeutendste erneuerbare Energie in Sachsen ablösen. Die weitere Nutzung dieser beiden Energiequellen stößt allerdings auf zunehmende ökologische Bedenken bzw. Widerstände.
Der Anteil der erneuerbaren Energiequellen am Elektroenergieverbrauch in Sachsen erreichte 1996 etwa 1,3 %. Bis zum Jahr 2000 erscheint eine Vergrößerung dieses Anteils auf ca. 5 % möglich.
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Forschungszentrum Rossendorf; FZR-193 August 1997
ISSN: 1436-3976
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Permalink: https://www.hzdr.de/publications/Publ-989
Publ.-Id: 989
Pre- and post-scission light charged particle multiplicities in incomplete fusion reactions
Yanez, R.
Abstract
In this article we present results concerning the extraction of light charged particle multiplicities in incomplete fusion-fission reactions with a moving source fitting procedure. To demonstrate the feasibility and reliability of the procedure we have used simulated events of known multiplicity to construct kinetic energy distributions at different angles that are fitted assuming several pre- and post-scission sources. In particular, we show that it is necessary to include at least two pre-equilibrium sources in order to extract correctly the known pre-equilibrium proton multiplicity. These two sources are characterized by high ernission temperatures, low emission barriers and high velocities, having ~ 70% and ~ 25% of the beam velocity along the beam axis, respectively The former source is naturally dominant at forward angles due to the strong focusing effect of its high velocity, Contrary to normal expectations, however, the slower pre-equilibrium source is present with considerable yield at the most backward angles θ ~ 145° where it is normally assumed only evaporative components are present. The estracted proton multiplicities are well reproduced by the moving source procedure, as well as fitting parameters with physical relevance.
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Forschungszentrum Rossendorf; FZR-192
ISSN: 1436-3976
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Permalink: https://www.hzdr.de/publications/Publ-988
Publ.-Id: 988
Test und Berechnung des passiven Notkondensators
Schaffrath, A.; Hicken, E. F.; Jaegers, H.; Prasser, H.-M.
The Siemens AG is developing the new innovative boiling water
reactor concept SWR1000. New features are the passive safety
systems (e.g. emergency condensers, building condensers, passive
pressure pulse transmitters).
For the experimental investigation of the emergency condenser
effectiveness, the NOKO test facility has been constructed at
the Forschungszentrum Jülich in cooperation with Siemens. The
facility has an operating pressure of 10 MPa and a maximum power
of 4 MW for steam production. The condenser bundle consists of 8
tubes and is fabricated with the geometry and material as planned
for the SWR. In more than 200 experiments, the emergency condenser
capacity was tested as a function of pressure, water level and
concentration of noncondensables in the pressure vessel as well as
pressure, water level and temperature in the condenser.
Posttest calculations of NOKO experiments were performed with an
improved version of ATHLET. To calculate the heat transfer coefficients
during condensation in horizontal tubes the module KONWAR has been
developed and implemented in ATHLET. KONWAR is based on the flow regime
map of Tandon and includes several semiempirical correlations for the
determination of the heat transfer coefficients. The presented comparison
between calculations and experiments shows a good agreement
- Atomwirtschaft-Atomtechnik 42 (1997), Nr. 11, S. 697-700
Permalink: https://www.hzdr.de/publications/Publ-986
Publ.-Id: 986
Analysis and Calculation of an Accident with Delayed Scram on NPP Greifswald Using the Coupled Code DYN3D/ATHLET
Kliem, S.
Analysis and calculation of an abnormal event which occurred in 1989 at the NPP Greifswald (VVER-440/213) are reported about. This event was a scram failure at about 50% nominal power with two of six working main coolant pumps (MCP). The analysis revealed remarkable differences between the active and passive loops due to non-homogeneous coolant mixing in the downcomer and lower plenum in the initial state before the accident. An existing input data deck for the coupled code DYN3D/ATHLET was modified to carry out calculations of this accident. On account of the absence of a mixing model considering loops with forward and loops with backward flow at the same time, the six reactor loops were modeled by a 3-fold (passive), a 2-fold (active) and a single (with the MCP to be switched-off at the beginning of the transient) loop. The comparison of the stationary calculation with the reported data shows a good agreement taking into account the mentioned deviations between the loops. Most of the calculated thermohydraulic parameters during the accident are very close to the measured data. Deviations in the loop temperatures can be explained by the differences in the measured stationary data and by the fact of non-homogeneous coolant mixing in the downcomer and the lower plenum. A small, but continuous power increase was observed during the whole time in the calculation while the measured power was remaining nearly constant. The power behaviour was brought into agreement with the measured data by a correction of the moderator temperature coefficient within the accuracy recommendations of the Atomic Energy Research (AER).
The calculation of this accident is an important contribution to the validation of the coupled code DYN3D/ATHLET. It demonstrated problems of the analysis of real abnormal events on NPP`s.
-
Contribution to proceedings
Proc. 7th Symposium of AER, pp.457-468, KFKI Atomic Energy Research Institute, Budapest (1997) -
Lecture (Conference)
7th Symposium of AER
Permalink: https://www.hzdr.de/publications/Publ-985
Publ.-Id: 985
Experimentelle Ergebnisse mit der NOKO-Versuchsanlage
Schaffrath, A.; Hicken, E. F.; Jaegers, H.; Prasser, H.-M.
On the NOKO (emergency condenser) test station constructed at Jülich Research Centre, the operating performance and effectiveness of the emergency condenser of the boiling water reactor 1000 have been determined in well over 200 tests. It has been possible to check that the tests were in close agreement with a modified version of ATHLET
- VGB-Kraftwerkstechnik 78 (1998), Heft 5, ISSN 0372-5715, S. 90-96
Permalink: https://www.hzdr.de/publications/Publ-984
Publ.-Id: 984
SANS Investigations of the Microstructure of VVER-440-Type RPV Steel after Low Temperature Irradiation at 60 grd C
Grosse, M.; Böhmert, J.; Gilles, R.
-
Poster
Annuals User's Meeting, Hahn-Meitner-Institut, Berlin, November 1997, Posterbeitrag
Permalink: https://www.hzdr.de/publications/Publ-983
Publ.-Id: 983
Perspektiven der Windenergienutzung in den neuen Bundesländern
Rindelhardt, U.
Der Stand und die Perspektiven der Windenergienutzung in den neuen Bundesländern unterscheidet sich nicht grundsätzlich von der Situation in den alten Ländern. In einigen Fragen (flächendeckende Potentialerhebungen, durchschnittliche WEA-Größe) ist der Stand sogar höher zu bewerten. Die weitere Entwicklung der Windenergienutzung wird bestimmt durch
- die mittelfristig mögliche Senkung der Stromgestehungskosten (Anforderungen an die Standortwahl und Standortnutzung),
- den praktischen Nachweis von Zuverlässigkeit und Lebensdauer der eingesetzten Anlagen,
- den künftigen ordnungspolitischen Rahmen für die Windenergienutzung (Zielkonflikt Liberalisierung der Strommärkte und Reduktion CO2-Ausstoß) sowie
- die politische und soziale Akzeptanz der Windenergienutzung.
Neben Wissenschaftlern und Technikern steht hier auch die Politik vor einer großen Herausforderung.
-
Lecture (Conference)
Tagungsband "Windenergienutzung im Binnenland", S. 168 -178 Kassel, 8./ 9. Oktober 1997 -
Contribution to proceedings
Tagungsband "Windenergienutzung im Binnenland", S. 168 -178 Kassel, 8./ 9. Oktober 1997
Permalink: https://www.hzdr.de/publications/Publ-982
Publ.-Id: 982
Definition of the Fifth Dynamic AER Benchmark Problem - A Benchmark for Coupled Thermohydraulic/ Three-Dimensional Hexagonal Neutron Kinetic Codes
Kliem, S.
The fifth dynamic benchmark defined in this paper is the first benchmark for coupled thermohydraulic system/three-dimensional neutron kinetic core models. In this benchmark the interaction between the components of a VVER-440 NPP with the reactor core should be investigated.
The initiating event is a symmetrical break of the main steam header (MSH) at the end of the first fuel cycle and hot shutdown conditions with one stuck out control rod group. The main purpose is the investigation of recriticality. For this reason, the calculation should be continued until the power excursion is eventually terminated by high-borated water from the high pressure injection system.
The participants of the benchmark should use own input data decks developed according to the needs of their own codes. The main geometrical parameters and characteristics of control and safety systems to be considered in this benchmark will be given to bring into agreement the data decks. Own best estimate nuclear cross section data should be used in the calculation. Only the initial subcriticality at the beginning of the transient will be given to made the results more comparable.
-
Contribution to proceedings
Proc. 7th Symposium of AER, pp.429-438 , KFKI Atomic Energy Research Institute, Budapest (1997) -
Lecture (Conference)
7th Symposium of AER
Permalink: https://www.hzdr.de/publications/Publ-981
Publ.-Id: 981
EXAFS Investigations of the Interaction of Humic Acids and Model Compounds with Uranyl Cations in Solid Complexes
Denecke, M. A.; Reich, T.; Pompe, S.; Bubner, M.; Heise, K.-H.; Nitsche, H.; Allen, P. G.; Bucher, J. J.; Edelstein, N. M.; Shuh, D. K.; Czerwinski, K.
-
Poster
Migration '97 Konferenz, 26.-31. Oktober, Sendai, Japan -
Radiochim. Acta 82, 103 (1998)
DOI: 10.1524/ract.1998.82.special-issue.103
Cited 32 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-980
Publ.-Id: 980
Bremsstrahlung in intermediate-energy nucleon reactions within an effective one-beson exchange model
Shklyar, V.; Kämpfer, B.; Reznik, B. L.; Titov, A. I.
Abstract
Within a covariant effective one-boson exchange model for the T matrix of NN interactions we present detailed calculations of bremsstrahlung cross sections for proton - proton and proton - neutron reactions at beam energies in the 1 GeV region. Besides pure bremsstrahlung processes we consider photons from ∆ decays and contributions from the η → γγ process. At beam energies above 700 MeV the ∆ decay channel dominates the spectra at large photon energies, where the interference between non-resonance processes and the ∆ decay channel becomes also important. Low energy photons stem from pure bremsstrahlung processes. The available experimental data at 730 MeV beam energy is well described. We extrapolate the model down to 280 MeV, where more detailed experimental data exist, and find agreement with angular distributions.
-
Forschungszentrum Rossendorf; FZR-191
ISSN: 1436-3976 - Nuclear Physics A 628 (1998) 255-274
Downloads
Permalink: https://www.hzdr.de/publications/Publ-979
Publ.-Id: 979
Precipitation Studies in Oxygen- and Nitrogen Rich Silicon Formed by High Dose Implantation
Weber, R.; Müller, R.; Skorupa, W.
-
Other report
E-MRS 1993 Spring Meeting, Strasbourg, May 4-7, 1993
DOI: 10.1016/0168-583X(94)95771-1
Cited 3 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-978
Publ.-Id: 978
CdS Nanocrystals Entrapped in Thin SiO2 Films
Pham, M. T.; Matz, W.; Möller, D.; Mücklich, A.; Oswald, S.
- Journal of Physical Chemistry B Vol. 102, Number 21, Pages 4081-4088, 1998
Permalink: https://www.hzdr.de/publications/Publ-977
Publ.-Id: 977
Correlation Between the Powder Structure and Microstructure of Tetragonal ZrO2 Ceramics
Haase, I.; Müller, R.
-
Poster
European Ceramic Society, Third Conference, Madrid, September 12-17, 1993, P04-05 (Poster)
Permalink: https://www.hzdr.de/publications/Publ-976
Publ.-Id: 976
Untersuchung der Wechselwirkungen zwischen ZrNb1 und austenitischem Stahl bei hohen Temperaturen
Müller, R.; Gleisberg, O.
-
Poster
29. Kolloquium des Arbeitskreises für Elektronenmikroskopische Direktabbildung und Analyse von Oberflächen (EDO) 8.-11. Oktober 1996 in Münster - Elektronenmikroskop. Direktabb. und Analyse v. Oberfl., 29 (1996)
Permalink: https://www.hzdr.de/publications/Publ-975
Publ.-Id: 975
Laserspektroskopie zur Bestimmung der chemischen Speziation von Uranylkomplexen
Bernhard, G.; Geipel, G.; Brendler, V.; Nitsche, H.
-
Poster
Poster bei der Hauptjahrestagung der GDCh, Wien, Sept. 1997
Permalink: https://www.hzdr.de/publications/Publ-974
Publ.-Id: 974
In-situ Laser Reflectometry Study of the Amorphization of Silicon Carbide by MeV Ion Implantation
Henkel, T.; Heera, V.; Kögler, R.; Skorupa, W.
-
Journal of Applied Physics,Vol 84, No. 6, Seite 3090-3097
DOI: 10.1063/1.368508
Cited 13 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-972
Publ.-Id: 972
Institute of Safety Research; Annual Report 1996
Weiß, F.-P.; Rindelhardt, U.; (Editors)
The report gives an overview on the scientific work of the Institute of Safety Research in 1996.
-
Forschungszentrum Rossendorf; FZR-190 August 1997
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-971
Publ.-Id: 971
Estimats of Dilepton Spectra from Open Charm and Bottom Decays in Relativistic Heavy-Ion Collisions
Kämpfer, B.; Pavlenko, O. P.
Abstract
The spectra of lepton pairs from correlated open charm and bottom decays in ultrarelativistic heavy-ion collisions are calculated. Our approach includes energy loss effects of the fast heavy quarks in deconfined matter which are determined by temperature and density of the expanding parton medium. We find a strong suppression of the initial transverse momentum spectrum of heavy quarks due to the energy lass at LHC conditions. Within the central rapidity covered by the ALICE detector system, the dominant contribution from bottom decays to the high invariant mass dielectron spectrum is predicted.
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Forschungszentrum Rossendorf; FZR-188
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-970
Publ.-Id: 970
Thermal Open Charm Signals Versus Hard Initial Yields in ultrarelativistic Heavy-Ion Collisions
Kämpfer, B.; Pavlenko, O. P.; Peshier, A.; Hentschel, M.; Soff, G.
Abstract.
Exploiting a unique set of parton distribution functions we estimate hard processes for open charm, dilepton and mini-jet production. Assuming rapid thermalization within the mini-jet plasma we follow the evolution (expansion and chemical equilibration) of the parton matter and calculate the energy loss of charm quarks in this environment. A substantial part of charm is espected to thermalize. We try to estimate the thermalized open charm component in the final hadron spectra.
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Journal of Physics G: Nucl. Part. Phys. 23 (1997) 2001-2011
DOI: 10.1088/0954-3899/23/12/025
Cited 36 times in Scopus -
Forschungszentrum Rossendorf; FZR-189
ISSN: 1436-3976
Permalink: https://www.hzdr.de/publications/Publ-969
Publ.-Id: 969
Investigation of Oxidation Resistance of Carbon Based First-Wall Liner Material Aerolor AO5
Krüssenberg, A.-K.; Moormann, R.; Hinssen, H.-K.; Hofmann, M.; Wu, C. H.
Minimizing the consequences of loss of vacuum and loss of coolant into vacuum accidents with respect to fusion reactor design requires the choice of materials as oxidation resistant as possible. In continuation to the testing of carbon candidate materials under oxidizing conditions (oxygen and steam) in collaboration with NET the carbon compound Aerolor AO5 of Carbone Lorraine has been examined in detail in the test facilities INDEX 2 and SPALEX at Forschungszentrum Jülich. The parameters for these oxidation experiments in the in-pore diffusion controlled regime are temperature (from 973 K up to 1173 K for oxygen, from 1173 K up to 1423 K for steam) and reaction gas concentration (1 vol.-% - 20 vol.% oxygen in argon, 5 vol.% - 100 vol.% steam in argon). The deducted equations for the primary oxidation reactions consider the dependence of the reaction rate on temperature, partial pressure and burn-off of the material.
-
Journal of Nuclear Materials 258-263 (1998) 770-776
DOI: 10.1016/S0022-3115(98)00256-6
Cited 4 times in Scopus -
Poster
Posterbeitrag während 8th International Conference Fusion Reactor Materials, 26.10 - 31.10.1997, Sendai, Japan
Permalink: https://www.hzdr.de/publications/Publ-968
Publ.-Id: 968
Studies of Liquid-Gaseous Two-Phase Systems by Positron Emitting Radiotracers
Hensel, F.
For a more detailed knowledge and understanding of various industrial processes an in-situ visualization is required. Positron Emission Tomography is an imaging technique used in medical research as a tool to study brain and heart diseases, allowing a non-invasive in-vivo concentration measurement of labeled substances. The mentioned features got us to carry out feasibility investigations for PET-like radiotracer applications in the field of two-phase flow systems. The main aim was to observe mixing and flow phenomena in efficient spatial and time resolution.
Typical values for the stopping ranges of positrons produced by common PET isotopes in water are approximately 2mm. Typical densities of the liquid-gaseous two phase systems that were to investigate are below 10% of the density of water under normal conditions. So the positron range effect becomes very important. Therefore as a first step the spatial annihilation distribution of a solid positron source has been measured using a Ti-45 source and solid blocks of polystyrene and polyurethane foam. The experiments have been carried out using a double head spherical PET-scanner for treatment plan verification of 3D conformable radiation therapy [1]. The foam density amounted from 15 kg/m3 to 38 kg/m3. The feasibility of a range based density measuring technique using the positron range was successfully shown. The next steps in this field could be the setup of a density measurement system for foams, including a detector optimization that results in an easy to handle low cost experimental assembly. It should comprise an encapsulated positron source and 2-4 pairs of detectors to cover an enlarged density range.
Liquid positron emitting tracers were used for monitoring phenomena in bubbly flows. PET experiments often require high activities and quite long integration times for an image reconstruction. Due to activity limitations it has been tried to optimize the experimental setup. Good results were achieved using a nearly two-dimensional geometry in combination with a midplane backprojection. In the experiments mixing processes in bubbly flows were observed using a F-18 solution. The bubbly flows were created by air injection. The event data were collected in list mode. The time resolution for these experiments was below 1s (integration time for the data evaluation). Best choice was a time step value of 500ms. In a further experiment the drainage of a surfactant stabilized foam was investigated.
Transport processes in bubbly flows and foams seem to be adequate topics for investigation using a PET technique. Time resolutions of about 1 s and below can be achieved, depending on the problem. The main advantage of PET tracers is the fact that many organic substances can be labeled with positron emitting isotopes which is important for the component sensitive investigation of many industrial processes.
-
Contribution to proceedings
3rd Topical Meeting on Industrial Radiation and Radioisotope Measurements and Applications, Conference Program and Abstracts, Raleigh, NC (USA), October 6-9, 1996, p. 101, ISBN 0-89448-645-2
DOI: 10.1016/S0969-8043(97)00144-9
Cited 6 times in Scopus - Applied Radiation and Isotopes 48 (1997), 1485 - 1492
-
Lecture (Conference)
3rd Topical Meeting on Industrial Radiation and Radioisotope Measurements and Applications, Raleigh, NC (USA), October 6-9, 1996
Permalink: https://www.hzdr.de/publications/Publ-967
Publ.-Id: 967
A numerical three-dimensional stability analysis of the MHD cylinder wake flow
Shatrov, V.; Mutschke, G.; Gerbeth, G.
-
Lecture (Conference)
3rd Int. Conference Transfer Phenomena in Magnetohydrodynamic and Electroconducting Flows; September 22-26, 1997 (Assois, France), Vol. 2, pp. 323 - 328 -
Contribution to proceedings
3rd Int. Conference Transfer Phenomena in Magnetohydrodynamic and Electroconducting Flows; September 22-26, 1997 (Assois, France), Vol. 2, pp. 323 - 328
Permalink: https://www.hzdr.de/publications/Publ-965
Publ.-Id: 965
Investigation of the Atomic Interdiffusion and Phase Formation in Ion Beam Irradiated Thin Cu-Al and Ag-Al Multilayers by In-situ RBS and XRD
Markwitz, A.; Matz, W.; Waldschmidt, U.; Demortier, G.
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Surface and Interface Analysis, Vol. 26, 160-174 (1998)
DOI: 10.1002/(SICI)1096-9918(199802)26:2<160::AID-SIA354>3.0.CO;2-M
Cited 8 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-964
Publ.-Id: 964
Test and Calculation of the Emergency Condenser of the SWR 1000
Schaffrath, A.; Prasser, H.-M.; Hicken, E. F.; Jaegers, H.
The Siemens AG is developing the new innovative boiling water reactor
concept SWR1000. New features are the passive safety systems (e.g.
emergency condensers, building condensers, passive pressure pulse
transmitters, gravitydriven core flooding lines).
For the experimental investigation of the emergency condenser effectiveness,
the NOKO test facility has been constructed at the Forschungszentrum Jülich
in cooperation with Siemens. This test facility has an operating pressure of
10 MPa and a maximum power of 4 MW for steam production. The emergency
condenser bundle consists of eight tubes and is fabricated with planned
geometry and material of the SWR1000. In more than 200 experiments, the
emergency condenser capacity was tested as a function of pressure, water
level and concentration of noncondensables in the pressure vessel as well
of pressure, water level and temperature in the condenser.
Post test calculations of NOKO experiments were performed with an improved
version of ATHLET. To calculate the heat transfer coefficients during
condensation in horizontal tubes the module KONWAR has been developed
and implemented in ATHLET. KONWAR is based on the flow regime map of
Tandon and includes several semiempirical correlations for the determination
of the heat transfer coefficients. The comparison between calculations and
experiments shows a good agreement.
-
Lecture (Conference)
Post-SMIRT 14 International Seminar "Passive Safety Features in Nuclear Installations", S B2.27-B2.35, 25.-27. August 1997, Pisa, Italien -
Contribution to proceedings
Post-SMIRT 14 International Seminar "Passive Safety Features in Nuclear Installations", S B2.27-B2.35, 25.-27. August 1997, Pisa, Italien
Permalink: https://www.hzdr.de/publications/Publ-963
Publ.-Id: 963
Non-destructive Evaluation of Glass Corrosion States
Mäder, M.; Grambole, D.; Herrmann, F.; Neelmeijer, C.; Schreiner, M.; Woisetschläger, G.
-
Nuclear Instruments and Methods in Physics Research B, 136-138 (1998) 863-868
DOI: 10.1016/S0168-583X(97)00749-0
Cited 20 times in Scopus -
Lecture (Conference)
13th Int. Conf. on Ion Beam Analysis (IBA-13), Lisboa, Portugal, July 27-Aug. 1, 1997
Permalink: https://www.hzdr.de/publications/Publ-962
Publ.-Id: 962
Modelling of boron nitride: atomic scale simulations on thin film growth
Albe, K.; Möller, W.
Molecular-dynamics simulations on ion-beam deposition
of boron nitride are presented. A realistic Tersoff-like potential energy
function for boron nitride, which was specially fitted to ab initio-data,
has been used. The impact of energetic boron and nitrogen atoms on a c-BN
target is simulated with energies ranging from 10 to 600 eV. The structural
analysis of the grown films shows, that a loose, dominantly sp2-bonded
structure arises at high ion flux. In no case the formation of a sp3-bonded
phase is observed, but the obtained films partially reveal textured basal
planes as found in experiment. Two different growth regimes are identified
for ion energies above and below 100 eV.
- Computational Materials Science 10 (1998) 111
-
Invited lecture (Conferences)
E-MRS Spring Meeting, Symp. D: Computational Modeling of Issues in Materials Science, Strasbourg, France, June 16 - 20, 1997 (invited lecture)
Permalink: https://www.hzdr.de/publications/Publ-961
Publ.-Id: 961
Preparation of SiO2 Films with embedded Si Nanocrystals by Reactive RF-Magnetron Sputtering
Seifarth, H.; Grötzschel, R.; Markwitz, A.; Matz, W.; Nitzsche, P.; Rebohle, L.
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Thin Solid Films 330 (1998) 202-205
DOI: 10.1016/S0040-6090(98)00609-9
Cited 68 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-960
Publ.-Id: 960
Increased Tool Cutling Life of Drills by Ion Implantation
Hilke, R.; Mändl, S.
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Other report
8th International DAAAM Symposium: Intelligent Manufacturing & Automation, Dubrovnik, Croatia, Oct. 28-25, 1997
Permalink: https://www.hzdr.de/publications/Publ-959
Publ.-Id: 959
Strömungsformen bei Kondensationsvorgängen im Notkondensator-Versuchsstand
Prasser, H.-M.; Böttger, A.; Schaffrath, A.
Im Rahmen des Forschungsvorhabens "Berechnung des passiven Notkondensators eines mit Naturumlauf arbeitenden innovativen Siedewasserreaktors (SWR600) mit ATHLET", das eng mit dem Forschungsvorhaben 15 NU 9050 "Notkondensator für einen Siedewasserreaktor mittlerer Leitung - Versuche zur Ermittlung der Leistung" verknüpft ist, wurden seitens des Forschungszentrums Rossendorf (FZR) e.V. im Rahmen eines F&E-Vertrages Auswertungen und Interpretationen von Messungen zu Strömungsformen und Kondensationsvorgängen im NOKO-Versuchsstand durchgeführt. Neben den Bündelversuchen wurden im NOKO-Versuchsstand mehrere Experimente im einem separaten, seitlich vom Bündel angeordneten und umfangreich instrumentierten Einzelrohr durchgeführt, um die Aussagesicherheit der Notkondensatorexperimente zu erhöhen und zusätzlich experimentelle Daten für die Validierung von Thermohydraulikprogrammsystemen (u. a. den ATHLET-Code) bereitzustellen. Hierbei geht es speziell um die Untersuchung der transienten Zweiphasenströmung innerhalb der Notkondensatorrohre hinsichtlich der dort anzutreffenden Strömungsformen, sowie die Bestimmung des volumentrischen Gasgehaltes an verschiedenen Stellen auf der Sekundärseite im Bündel bei unterkühltem und gesättigtem Sieden. Das NOKO-Einzelrohr wurde hierzu mit nadelförmigen Voidsonden ausgestattet. Durch die Nutzung von jeweils mehreren Sonden in zwei ausgewählten Strömungsquerschnitten wurde die Phasenverteilung während der Füllstandsabsenkung, d.h. beim Durchgang des Flüssigkeitsspiegels an den Sondenpositionen, in-stationär gemessen. Daraus läßt sich die Form der Phasengrenzfläche rekonstruieren. Neben den Messungen im Einzelrohr fanden, ebenfalls mit Nadelsonden, Messungen auf der Sekundärseite des NOKO-Bündels statt. Die Einzelrohr-Versuche an der NOKO-Anlage in Jülich haben gezeigt daß bei entsprechend geringer Konzentration von nichtkondensierbaren Gasen Schwälle und Pfropfen im Ansatz zu beobachten sind, die Vorhersagen bekannter Strömungskarten jedoch nicht zutreffen. Dort werden Schwälle und Pfropfen in wesentlich größerem Aumaß vorhergesagt. Die Aufstellung und Validierung eines einfachen Modells zur Berechnung des Druckverlustes im Wärmeübertragerrohr ist gelungen. Damit kann der Differenzdruck zwischen den Kollektoren ober besser ein an den Wärmeübertragerrohren direkt gemessener Differenzdruck zur Füllstandsmessung auf der Primärseite des Notkondensators herangezogen werden. Bei der Validierung mußten jedoch die experimentell ermittelten Volumina des nichtkondensierbaren Gases in die Berechnung einfließen. Der Mechanismus der Kondensationsbehinderung durch das nichtkondensierbare Gas wurde durch Gegenüberstellung der Sondendaten mit den Meßwerten der Thermoelemente im Einzelrohr im Detail untersucht.
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Wissenschaftlich-Technische Berichte / Forschungszentrum Rossendorf; FZR-186 Juli 1997
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-958
Publ.-Id: 958
Analysis of deuterium induced nuclear reactions giving criteria for the formation process of expanded austenite
Parascandola, S.; Günzel, R.; Grötzschel, R.; Richter, E.; Möller, W.
High current ion nitriding of austenitic stainless steel at temperatures of about 400°C leads to the formation of a surface layer, called expanded austenite. The formation of this layer is not well understood. Deuterium induced nuclear reaction analyses have been performed on austenitic stainless steel samples that were subsequently high current ion nitrided with low energy ion implantation of 15 N and 14 N. The obtained depth profiles yield criteria for the formation process of the expanded austenite. A trapping mechanism cannot be confirmed.
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Nuclear Instruments and Methods in Physics Research B, 136-138 (1998) 1281
DOI: 10.1016/S0168-583X(97)00844-6
Cited 39 times in Scopus - Poster und Beitrag zu Sammelwerken / Proceedings of the Thirteenth International Conference on Ion Beam Analysis, Lisbon, Portugal, 27 July - 1 August 1997
Permalink: https://www.hzdr.de/publications/Publ-956
Publ.-Id: 956
Comment on "On the Relation Between Unimolekular Reaction Rates and Overlapping Resonances"
Rotter, I.
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J. Chem. Phys. 106(11), 4810, 15 March 1997
DOI: 10.1063/1.473989
Permalink: https://www.hzdr.de/publications/Publ-955
Publ.-Id: 955
Initial Inter-Laboratory Testing of the Rossendorf-Oxford (ROX97) Secondary Standard for X-ray Analysis
Neelmeijer, C.; Mäder, M.; Jarjis, R.; Calligaro, T.; Salomon, J.; Schreiner, M.; Gantz, T.
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Nuclear Instruments and Methods in Physics Research B, 136-138 (1998) 902-907
DOI: 10.1016/S0168-583X(97)00821-5
Cited 2 times in Scopus -
Lecture (Conference)
13. Int. Conf. on Ion Beam Analysis (IBA-13), Lisboa, Portugal, July 27 - Aug. 1, 1997
Permalink: https://www.hzdr.de/publications/Publ-954
Publ.-Id: 954
Estimates of Dilepton Spectra from Open Charm and Bottom Decays in Relativistic Heavy-Ions Collisions
Kämpfer, B.; Pavlenko, O. P.; Gallmeister, K.
-
Physics Letters B 419 (1998) 412-418
DOI: 10.1016/S0370-2693(97)01469-X
Cited 22 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-953
Publ.-Id: 953
Determination of Structural Parameters of Uranyl Ion Complexed with Organic Acids Using EXAFS
Denecke, M. A.; Reich, T.; Bubner, M.; Heise, K.-H.; Nitsche, H.; Allen, P. G.; Bucher, J. J.; Edelstein, N. M.; Shuh, D. K.
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Contribution to external collection
Actinides '97 Conf. -
J. Alloys and Compounds 271-273, 123 (1998)
DOI: 10.1016/S0925-8388(98)00038-3
Cited 51 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-952
Publ.-Id: 952
Synthetische Huminsäuren für die Umweltforschung
Heise, K.-H.; Pompe, S.; Bubner, M.; Nitsche, H.
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Lecture (Conference)
Arbeitstagung der Deutschen Gesellschaft für Moor- und Torfkunde e. V., Bad Elster, Germany, 04.-05.09. 1997
Permalink: https://www.hzdr.de/publications/Publ-951
Publ.-Id: 951
LOWRAD 96; Methods and Applications of Low-Level Radioactivity Measurements; Proceedings of a Workshop Rossendorf/Dresden, 7-8 November 1996
Nitsche, H.; Niese, S.
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Forschungszentrum Rossendorf; FZR-170
ISSN: 1436-3976
Downloads
Permalink: https://www.hzdr.de/publications/Publ-948
Publ.-Id: 948
Nuclear and Hadron Physics and Project ELBE; Annual Report 1996
Barz, H.-W.; Dönau, F.; Enghardt, W.; Grosse, E.; Kämpfer, B.; Prade, H.; Schlett, M.; Wünsch, R.
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Forschungszentrum Rossendorf; FZR-179 April 1997
ISSN: 1436-3976
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Permalink: https://www.hzdr.de/publications/Publ-947
Publ.-Id: 947
The Chiral Quark-Loop Soliton in a Hot Gas of Constituent Quarks
Schleif, M.; Wünsch, R.
Abstract
We consider a chiral one-loop hedgehog soliton of the bosonized SU(2)f Nambu & Jona-Lasinio model which is embedded in a liot medium of constituent quarks. Energy and radius of the soliton are determined in self-consistent mean-field approximation. Quasi-classical corrections to the soliton energy are derived by means of the pushing and cranking approaches. The corresponding inertial parameters are evaluated. It is shown that the inertial mass is equivalent to the total internal energy of the soliton. Corrected nucleon and ∆ isobar masses are calculated in dependence on temperature and density of the medium. As a result of the internal structure of the soliton which is controlled by the self-consistent mean field, the scaling between constituent quark mass and soliton mass is noticeable disturbed.
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Forschungszentrum Rossendorf; FZR-182
ISSN: 1436-3976
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Permalink: https://www.hzdr.de/publications/Publ-946
Publ.-Id: 946
Ionendriftprozesse in Borsilikatgläsern während des anodischen Bondens
Nitzsche, P.; Lange, K.; Schmidt, B.; Grigull, S.; Kreißig, U.; Huber, H.; Assmann, W.; Thomas, B.; Herzog, K.
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Forschungszentrum Rossendorf; FZR-184 Juli 1997
ISSN: 1436-3976
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Permalink: https://www.hzdr.de/publications/Publ-944
Publ.-Id: 944
N.C.A.11C-Labelling of Benzenoid Compounds in Ring Positions: [11C]Anisole Derivatives
Mäding, P.; Steinbach, J.; Johannsen, B.
The synthesis route to n.c.a. 3-nitro-[3-C-11]anisole (3) by use of the principle of synchronous six-electron cyclization of hexatriene systems into aromatics is described and discussed. Nitro-[C-11]-methane (1) reacts with the prepared precursor 5-dimethylamino-2-methoxy-penta-2,4-dienylidene-1-dimethylammonium tetrafluoroborate (2b) in the presence of BuLi to form 1-dimethylamino-4-methoxy-6-nitro-[6-C-11]hexatriene (IA, IB), followed by cyclization/ aromatization into 3. Starting from 1, 3-nitro-[3-C-11]anisole of a radiochemical purity of about 65 % and a mean specific radioactivity of 1 Ci/mu mol was obtained within 10 min. Related to [C-11]CH3NO2, the reproducible radiochemical yield of 3 (decay-corrected) was 60+/-5 %. Reduction of 3 by heating the above reaction mixture with aqueous Na2S gave 3-amino-[3-C-11]anisole (4) of a radiochemical purity of about 50 %. The reproducible radiochemical yield of 4 (decay-corrected) in relation to 1 was 45+/-5 %, the synthesis time from 1 was 16 min.
- Journal of Labelled Compounds and Radiopharmaceuticals 39 (7): 585-599 JUL 1997
Permalink: https://www.hzdr.de/publications/Publ-942
Publ.-Id: 942
Sheath and Presheath Dynamics in Plasma Immersion Ion Implantation
Mändl, S.; Günzel, R.; Möller, W.
- Journal of Physics D: Applied Physics 31 (1998) 1109-1117
Permalink: https://www.hzdr.de/publications/Publ-940
Publ.-Id: 940
Helium Bubbles in Silicon: Study of the Residual Helium Content using Elastic Recoil Detection Analysis
Kaschny, J. R.; Fichtner, P. F. P.; Mücklich, A.; Kreißig, U.; Yankov, R. A.; Skorupa, W.
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Lecture (Conference)
13th Int. Conf. on Ion Beam Analysis (IBA-13), Lissabon, Portugal, July 27 - Aug 1, 1997 -
Contribution to external collection
Nucl. Instr. Meth. B136-138 (1998) 583
Permalink: https://www.hzdr.de/publications/Publ-939
Publ.-Id: 939
Identification and Discrimination of Thiobacilli Using ARDREA, RAPD and Rep-APD
Selenska-Pobell, S.; Otto, A.; Kutschke, S.
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Journal of Applied Bacteriology, 84, (1998), p. 1085-1091
DOI: 10.1046/j.1365-2672.1998.00444.x
Cited 33 times in Scopus -
Poster
15. DECHEMA-Jahrestagung der Biotechnologen, Münster, 04.-06.03.1997
Permalink: https://www.hzdr.de/publications/Publ-938
Publ.-Id: 938
In Situ ERDA Studies of Ion Drift Processes
Kreißig, U.; Grigull, S.; Lange, K.; Nitzsche, P.; Schmidt, B.
- Nuclear Instruments and Methods in Physics Research B ( IBA '97)
Permalink: https://www.hzdr.de/publications/Publ-937
Publ.-Id: 937
Angle dependent Mössbauer Spectroscopy
Reuther, H.; Behr, G.
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Contribution to external collection
Hyperfine Interactions ( ICAME '97 Conf. Proc.)
Permalink: https://www.hzdr.de/publications/Publ-936
Publ.-Id: 936
Alloying by High Dose Ion Implantation of Iron into Magnesium and Aluminium
Reuther, H.; Betzl, M.; Matz, W.; Richter, E.
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Hyperfine Interactions 113 (1998) 391-401
DOI: 10.1023/A:1012648321780
Permalink: https://www.hzdr.de/publications/Publ-935
Publ.-Id: 935
Phase Formation of Iron Silicides by Ion Implantation
Dobler, M.; Reuther, H.; Möller, W.
- Hyperfine Interactions (C) 3 (1998) 145-148
Permalink: https://www.hzdr.de/publications/Publ-934
Publ.-Id: 934
A Combination of Atomic and Continuum Models Describing the Evolution of Nanoclusters
Strobel, M.; Heinig, K.-H.; Möller, W.
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Computational Materials Science 10 (1998) 457-462
DOI: 10.1016/S0927-0256(97)00114-6
Cited 11 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-933
Publ.-Id: 933
Molecular-Dynamics Studies of a C:H Film Growth by Energetic Hydrocarbon Molecule Impact
Jäger, H.-U.; Weiler, W.
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Diamond and Related Materials 7 (1998) 858-863
DOI: 10.1016/S0925-9635(97)00314-2
Cited 10 times in Scopus -
Lecture (Conference)
8th European Conference on Diamond, Diamond-Like and Related Materials, Edinburgh, UK, Aug. 3 - 8, 1997
Permalink: https://www.hzdr.de/publications/Publ-931
Publ.-Id: 931
Novel Rhenium Complexes Derived from ALPHA-Tropanol as Potential Ligands for the Dopamin Transporter
Hoepping, A.; Brust, P.; Berger, R.; Leibnitz, P.; Spies, H.; Machill, S.; Scheller, D.; Johannsen, B.
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Bioorganic & Medicinal Chemistry 6 (1998) 1663-1672
DOI: 10.1016/S0968-0896(98)00144-8
Cited 11 times in Scopus
Permalink: https://www.hzdr.de/publications/Publ-930
Publ.-Id: 930
Pages: [1.] [2.] [3.] [4.] [5.] [6.] [7.] [8.] [9.] [10.] [11.] [12.] [13.] [14.] [15.] [16.] [17.] [18.] [19.] [20.] [21.] [22.] [23.] [24.] [25.] [26.] [27.] [28.] [29.] [30.] [31.] [32.] [33.] [34.] [35.] [36.] [37.] [38.] [39.] [40.] [41.] [42.] [43.] [44.] [45.] [46.] [47.] [48.] [49.] [50.] [51.] [52.] [53.] [54.] [55.] [56.] [57.] [58.] [59.] [60.] [61.] [62.] [63.] [64.] [65.] [66.] [67.] [68.] [69.] [70.] [71.] [72.] [73.] [74.] [75.] [76.] [77.] [78.] [79.] [80.] [81.] [82.] [83.] [84.] [85.] [86.] [87.] [88.] [89.] [90.] [91.] [92.] [93.] [94.] [95.] [96.] [97.] [98.] [99.] [100.] [101.] [102.] [103.] [104.] [105.] [106.] [107.] [108.] [109.] [110.] [111.] [112.] [113.] [114.] [115.] [116.] [117.] [118.] [119.] [120.] [121.] [122.] [123.] [124.] [125.] [126.] [127.] [128.] [129.] [130.] [131.] [132.] [133.] [134.] [135.] [136.] [137.] [138.] [139.] [140.] [141.] [142.] [143.] [144.] [145.] [146.] [147.] [148.] [149.] [150.] [151.] [152.] [153.] [154.] [155.] [156.] [157.] [158.] [159.] [160.] [161.] [162.] [163.] [164.] [165.] [166.] [167.] [168.] [169.] [170.] [171.] [172.] [173.] [174.] [175.] [176.] [177.] [178.] [179.] [180.] [181.] [182.] [183.] [184.] [185.] [186.] [187.] [188.] [189.] [190.] [191.] [192.] [193.] [194.] [195.] [196.] [197.] [198.] [199.] [200.] [201.] [202.] [203.] [204.] [205.] [206.] [207.] [208.] [209.] [210.] [211.] [212.] [213.] [214.] [215.] [216.] [217.] [218.] [219.] [220.] [221.] [222.] [223.] [224.] [225.] [226.] [227.] [228.] [229.] [230.] [231.] [232.] [233.] [234.] [235.] [236.] [237.] [238.] [239.] [240.] [241.] [242.] [243.] [244.] [245.] [246.] [247.] [248.] [249.] [250.] [251.] [252.] [253.] [254.] [255.] [256.] [257.] [258.] [259.] [260.] [261.] [262.] [263.] [264.] [265.] [266.] [267.] [268.] [269.] [270.] [271.] [272.] [273.] [274.] [275.] [276.] [277.] [278.] [279.] [280.] [281.] [282.] [283.] [284.] [285.] [286.] [287.] [288.] [289.] [290.] [291.] [292.] [293.] [294.] [295.] [296.] [297.] [298.] [299.] [300.] [301.] [302.] [303.] [304.] [305.] [306.] [307.] [308.] [309.] [310.] [311.] [312.] [313.] [314.] [315.] [316.] [317.] [318.] [319.] [320.] [321.] [322.] [323.] [324.] [325.] [326.] [327.] [328.] [329.] [330.] [331.] [332.] [333.]